Mechanism analysis and mixing characterization of variable-speed mechanical mixing enhancement

IF 1.6 4区 工程技术 Q3 Chemical Engineering International Journal of Chemical Reactor Engineering Pub Date : 2024-04-19 DOI:10.1515/ijcre-2023-0239
Yuchen Lin, Shibo Wang, Hua Wang, Jianxin Xu, Q. Xiao
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Abstract

In response to the observed phenomenon of poor fluid mixing within the reactor, this study proposes a novel mixing method to enhance fluid mixing efficiency. In this study, numerical simulation and purification tests were carried out for the purification of zinc sulfate solution. Numerical simulations were conducted to compare the effects of variable-speed stirring and uniform-speed stirring on mixing efficiency, considering both momentum transfer process and mass transfer process. The purification test further demonstrated a significant improvement in the reaction rate under variable-speed stirring, as evidenced by the analysis of purification efficiency and microscopic morphology. It was elaborated that the enhancement mechanism of variable-speed stirring involved disrupting the periodic order structure in the tank, leading to the generation of a multi-scale vortex that increased stirring kinetic energy to form a shear force. This force contributed to reducing the velocity slip between the impurity ions and zinc particles, consequently decreasing reaction time and enhancing purification rate. The results indicated that sinusoidal stirring yielded the most effective mixing. When implemented in practical production settings, it enhanced dimensionless mixing efficiency by 24.83 % compared to the homogeneous stirring system. Additionally, it reduced reaction time by 15.47 % and decreased mixing energy per unit volume by 32.38 %, while simultaneously lowering energy consumption by 24.77 %.
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变速机械搅拌的机理分析和搅拌特性分析
针对观察到的反应器内流体混合不良的现象,本研究提出了一种新型混合方法,以提高流体混合效率。本研究针对硫酸锌溶液的净化进行了数值模拟和净化试验。数值模拟比较了变速搅拌和匀速搅拌对混合效率的影响,同时考虑了动量传递过程和质量传递过程。净化试验进一步证明了变速搅拌下反应速率的显著提高,净化效率和微观形态分析也证明了这一点。研究阐述了变速搅拌的增强机理,即破坏槽内的周期性有序结构,产生多尺度涡流,增加搅拌动能,形成剪切力。这种剪切力有助于减少杂质离子和锌颗粒之间的速度滑移,从而缩短反应时间,提高纯化率。结果表明,正弦搅拌产生的混合效果最好。在实际生产中,与均匀搅拌系统相比,正弦搅拌的无量纲混合效率提高了 24.83%。此外,它还将反应时间缩短了 15.47%,将单位体积的搅拌能量降低了 32.38%,同时将能耗降低了 24.77%。
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来源期刊
CiteScore
2.80
自引率
12.50%
发文量
107
审稿时长
3 months
期刊介绍: The International Journal of Chemical Reactor Engineering covers the broad fields of theoretical and applied reactor engineering. The IJCRE covers topics drawn from the substantial areas of overlap between catalysis, reaction and reactor engineering. The journal is presently edited by Hugo de Lasa and Charles Xu, counting with an impressive list of Editorial Board leading specialists in chemical reactor engineering. Authors include notable international professors and R&D industry leaders.
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