{"title":"Subpicosecond laser ablation behavior of magnesium target and crater evolution: Molecular dynamics study and experimental validation","authors":"Guo-hsiang Jiang, Xia Zhou","doi":"10.1088/1674-1056/ad3ef8","DOIUrl":null,"url":null,"abstract":"\n The micro-ablation processes and morphology evolution of ablative craters on single-crystal magnesium under subpicosecond laser irradiation are investigated by MD simulations and experiments. Simulation results exhibit that the main failure mode of single-crystal Mg film irradiated by low fluence and long width pulse laser is the ejection of surface atoms which have laser-induced high stress. But under high fluence and short width pulse laser irradiation, the main damage mechanism is nucleation fracture caused by stress wave reflection and superposition at the bottom of the film. In addition, Mg[0001] has higher pressure sensitivity and is more prone to ablation than Mg[1010].The evolution equation of crater depth was established by the multi-pulse laser ablation simulation and verified by experiments. The results show that, under multiple pulsed laser irradiation, not only crater depth increases linearly with the pulse number, but also the quadratic term and constant term of the fitted crater profile curve increase linearly.","PeriodicalId":1,"journal":{"name":"Accounts of Chemical Research","volume":"82 2","pages":""},"PeriodicalIF":17.7000,"publicationDate":"2024-04-16","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Accounts of Chemical Research","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1088/1674-1056/ad3ef8","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The micro-ablation processes and morphology evolution of ablative craters on single-crystal magnesium under subpicosecond laser irradiation are investigated by MD simulations and experiments. Simulation results exhibit that the main failure mode of single-crystal Mg film irradiated by low fluence and long width pulse laser is the ejection of surface atoms which have laser-induced high stress. But under high fluence and short width pulse laser irradiation, the main damage mechanism is nucleation fracture caused by stress wave reflection and superposition at the bottom of the film. In addition, Mg[0001] has higher pressure sensitivity and is more prone to ablation than Mg[1010].The evolution equation of crater depth was established by the multi-pulse laser ablation simulation and verified by experiments. The results show that, under multiple pulsed laser irradiation, not only crater depth increases linearly with the pulse number, but also the quadratic term and constant term of the fitted crater profile curve increase linearly.
期刊介绍:
Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance.
Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.