MALTA: A Zonally Averaged Global Atmospheric Transport Model for Long-Lived Trace Gases

IF 4.4 2区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Journal of Advances in Modeling Earth Systems Pub Date : 2024-05-02 DOI:10.1029/2023MS003909
Luke M. Western, Scott D. Bachman, Stephen A. Montzka, Matt Rigby
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Abstract

We present a two-dimensional, zonally averaged global model of atmospheric transport named MALTA: Model of Averaged in Longitude Transport in the Atmosphere. It aims to be accessible to a broad community of users, with the primary function of quantifying emissions of greenhouse gases and ozone depleting substances. The model transport is derived from meteorological reanalysis data and flux-gradient experiments using a three-dimensional transport model. Atmospheric sinks are prescribed loss frequency fields. The zonally averaged model simulates important large-scale transport features such as the influence on trace gas concentrations of the quasi-biennial oscillation and variations in inter-hemispheric transport rates. Stratosphere-troposphere exchange is comparable to a three-dimensional model and inter-hemispheric transport is faster by up to 0.3 years than typical transport times of three-dimensional models, depending on the metric used. Validation of the model shows that it can estimate emissions of CFC-11 from an incorrect a priori emissions field well using three-dimensional (3D) mole fraction fields generated using a different 3D model than which the flux gradient relationships were derived. The model is open source and is expected to be applicable to a wide range of studies requiring a fast, simple model of atmospheric transport and chemical processes for estimating associated emissions or mole fractions.

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MALTA:长寿命痕量气体分区平均全球大气传输模型
我们提出了一个二维分区平均全球大气传输模型,命名为 MALTA:大气经度平均传输模型。该模型旨在供广大用户使用,主要功能是量化温室气体和臭氧消耗物质的排放。模型传输来自气象再分析数据和使用三维传输模型的通量梯度实验。大气汇是规定的损失频率场。分区平均模型模拟了重要的大尺度传输特征,如准双年振荡对痕量气体浓度的影响以及半球间传输速率的变化。同温层与对流层的交换与三维模型相当,而半球间的传输速度比三维模型的典型传输速度快 0.3 年,这取决于所使用的指标。对模型的验证表明,该模型可以很好地利用不同的三维模型生成的三维(3D)分子分数场,从一个不正确的先验排放场估算出 CFC-11 的排放量,而通量梯度关系是通过该模型推导出来的。该模型是开放源码的,预计将适用于需要快速、简单的大气传输和化学过程模型来估算相关排放量或摩尔分数的各种研究。
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来源期刊
Journal of Advances in Modeling Earth Systems
Journal of Advances in Modeling Earth Systems METEOROLOGY & ATMOSPHERIC SCIENCES-
CiteScore
11.40
自引率
11.80%
发文量
241
审稿时长
>12 weeks
期刊介绍: The Journal of Advances in Modeling Earth Systems (JAMES) is committed to advancing the science of Earth systems modeling by offering high-quality scientific research through online availability and open access licensing. JAMES invites authors and readers from the international Earth systems modeling community. Open access. Articles are available free of charge for everyone with Internet access to view and download. Formal peer review. Supplemental material, such as code samples, images, and visualizations, is published at no additional charge. No additional charge for color figures. Modest page charges to cover production costs. Articles published in high-quality full text PDF, HTML, and XML. Internal and external reference linking, DOI registration, and forward linking via CrossRef.
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