Uncovering the dynamics of atmospheric aerosols in China: A comprehensive analysis of OMI-Retrieved aerosol index data

IF 1.8 4区 地球科学 Q3 GEOCHEMISTRY & GEOPHYSICS Journal of Atmospheric and Solar-Terrestrial Physics Pub Date : 2024-04-30 DOI:10.1016/j.jastp.2024.106251
Muhammad Khan , Salman Tariq
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Abstract

China faces severe atmospheric problems due to the rapid increase in population and industrialization. Therefore, due to the insufficient number of monitoring stations in such a vast country, remote sensing of an ultraviolet aerosol index (UVAI) provides useful information about absorbing aerosols. This study used the OMI-retrieved UVAI data to investigate the spatial patterns, trends, and periodic nature of UVAI over China from October 2004 to December 2022. Additionally, the correlation and degree of coherence of UVAI with meteorological parameters (temperature & precipitation) and anthropogenic factors (Construction, population, CO2 emission, energy consumption, and primary industry) are also examined. Mean UVAI concentration with an increasing trend of 4.34% per year shows high UVAI values (0.70–1.41) in Xinjiang Uygar followed by Heilongjiang, Jilin, Liaoning, Shandong, Beijing, Hubei, and some northern regions i.e., Gansu, Qinghai, and western Nel Mongol. Seasonally, Xinjiang Uygur experiences high UVAI (<1.52) values during all four seasons with the dominance of both fine and coarse mode particles. Moreover, Hubei, Gansu, Jilin, Shandong, and Xinjiang Uygar experiences high UVAI values i.e. 2.55, 2.05, 1.87, 2.82, 2.27 during 2021 with an increasing trend of 5.50% year−1, 5.43% year−1, 3.82% year−1, 4.73% year−1, and 9.33% year−1 respectively. The HYSPLIT backward trajectories plotted at altitudes of 50m, 100m, and 500m indicate the dominance of desert dust over Jinan, Urumqi, and Lanzhou while anthropogenic pollutants over Wuhan and Changchun. Wavelet coherence (WTC) shows the positive correlation of UVAI with temperature and precipitation. Moreover, the co-variability of absorbing aerosols with anthropogenic and natural factors is also inculcated in this study. Considering the outcomes of this study it will help policymakers to analyze the variability of absorbing aerosols in China and different methods like plantation of more trees, efficient fuel consumption, and promotion of public transport, etc., can be used to reduce air pollution.

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揭示中国大气气溶胶的动态变化:OMI 气溶胶指数数据的综合分析
由于人口和工业化的快速发展,中国面临着严重的大气问题。因此,在这样一个幅员辽阔的国家,由于监测站点数量不足,紫外线气溶胶指数(UVAI)遥感提供了有关吸收气溶胶的有用信息。本研究利用 OMI 检索到的紫外气溶胶指数数据,研究了 2004 年 10 月至 2022 年 12 月中国上空紫外气溶胶指数的空间模式、趋势和周期性。此外,还研究了 UVAI 与气象参数(气温 & 降水)和人为因素(建筑、人口、二氧化碳排放、能源消耗和第一产业)的相关性和一致性。结果表明,新疆维吾尔自治区的紫外辐射平均值较高(0.70-1.41),其次是黑龙江、吉林、辽宁、山东、北京、湖北,以及北方的甘肃、青海和内蒙古西部地区。从季节上看,新疆维吾尔自治区四季都有较高的 UVAI 值(1.52),细颗粒物和粗颗粒物都占优势。此外,湖北、甘肃、吉林、山东和新疆维吾尔自治区在 2021 年的 UVAI 值也较高,分别为 2.55、2.05、1.87、2.82 和 2.27,且呈逐年上升趋势,分别为 5.50%、5.43%、3.82%、4.73% 和 9.33%。在 50 米、100 米和 500 米高度绘制的 HYSPLIT 后向轨迹表明,济南、乌鲁木齐和兰州上空以沙漠沙尘为主,而武汉和长春上空则以人为污染物为主。小波相干性(WTC)表明 UVAI 与温度和降水呈正相关。此外,吸收气溶胶与人为和自然因素的共同可变性也在本研究中得到了体现。考虑到这项研究的结果,它将有助于决策者分析中国吸收性气溶胶的可变性,并采用不同的方法,如种植更多树木、高效燃料消耗和推广公共交通等,以减少空气污染。
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来源期刊
Journal of Atmospheric and Solar-Terrestrial Physics
Journal of Atmospheric and Solar-Terrestrial Physics 地学-地球化学与地球物理
CiteScore
4.10
自引率
5.30%
发文量
95
审稿时长
6 months
期刊介绍: The Journal of Atmospheric and Solar-Terrestrial Physics (JASTP) is an international journal concerned with the inter-disciplinary science of the Earth''s atmospheric and space environment, especially the highly varied and highly variable physical phenomena that occur in this natural laboratory and the processes that couple them. The journal covers the physical processes operating in the troposphere, stratosphere, mesosphere, thermosphere, ionosphere, magnetosphere, the Sun, interplanetary medium, and heliosphere. Phenomena occurring in other "spheres", solar influences on climate, and supporting laboratory measurements are also considered. The journal deals especially with the coupling between the different regions. Solar flares, coronal mass ejections, and other energetic events on the Sun create interesting and important perturbations in the near-Earth space environment. The physics of such "space weather" is central to the Journal of Atmospheric and Solar-Terrestrial Physics and the journal welcomes papers that lead in the direction of a predictive understanding of the coupled system. Regarding the upper atmosphere, the subjects of aeronomy, geomagnetism and geoelectricity, auroral phenomena, radio wave propagation, and plasma instabilities, are examples within the broad field of solar-terrestrial physics which emphasise the energy exchange between the solar wind, the magnetospheric and ionospheric plasmas, and the neutral gas. In the lower atmosphere, topics covered range from mesoscale to global scale dynamics, to atmospheric electricity, lightning and its effects, and to anthropogenic changes.
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