Projected changes in ultraviolet index and UV doses over the twenty-first century: impacts of ozone and aerosols from CMIP6.

IF 2.7 3区 化学 Q3 BIOCHEMISTRY & MOLECULAR BIOLOGY Photochemical & Photobiological Sciences Pub Date : 2024-07-01 Epub Date: 2024-05-19 DOI:10.1007/s43630-024-00594-7
Ana Letícia Campos Yamamoto, Marcelo de Paula Corrêa, Roger Rodrigues Torres, Fabrina Bolzan Martins, Sophie Godin-Beekmann
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Abstract

This study evaluated the health-related weighted ultraviolet radiation (UVR) due to the total ozone content (TOC) and the aerosol optical depth (AOD) changes. Clear-sky Ultraviolet Index (UVI), daily doses, and exposure times for erythema induction (Dery and Tery) and vitamin D synthesis (DvitD and TvitD) were computed by a radiative transfer estimator. TOC and AOD data were provided by six Earth System Models (ESMs) from the Coupled Model Intercomparison Project Phase 6 (CMIP6). For projections, we consider four Shared Socioeconomic Pathways scenarios-SSPs (SSP1-2.6, SSP2-4.5, SSP3-7.0, and SSP5-8.5)-and two time-slices (near: 2041-2060 and far future: 2081-2100). UVR projections showed pronounced changes for the summer hemispheres in the far future. TOC increases in mid- and high latitudes of the Southern Hemisphere caused decreases in UVR at the summer solstice. However, projections did not indicate sun-safe exposure conditions in South America, Australia, and Southern Africa. On the contrary, exposure around solar noon from 10 to 20 min will still be sufficient to induce erythema in skin type III individuals throughout this century. In southern Argentina and Chile, the UVR insufficiency for vitamin D synthesis at solar noon in skin type III remains the same during this century at the winter solstice. In the Northern Hemisphere, UVI and Dery at the summer solstice should remain high (UVI ≥ 8; Dery ~ 7.0 kJ m-2) in highly populated locations. Above 45 °N, UVR levels cannot be enough to synthesize vitamin D in skin type III during the boreal winter. Our results show that climate change will affect human health through excess or lack of solar UVR availability.

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预测二十一世纪紫外线指数和紫外线剂量的变化:CMIP6 中臭氧和气溶胶的影响。
本研究评估了臭氧总含量(TOC)和气溶胶光学深度(AOD)变化引起的与健康相关的加权紫外线辐射(UVR)。晴空紫外线指数(UVI)、每日剂量以及红斑诱导(Dery 和 Tery)和维生素 D 合成(DvitD 和 TvitD)的照射时间均由辐射传递估算器计算得出。TOC和AOD数据由耦合模式相互比较项目第六阶段(CMIP6)的六个地球系统模式(ESM)提供。在预测时,我们考虑了四种共享社会经济路径情景(SSP1-2.6、SSP2-4.5、SSP3-7.0 和 SSP5-8.5)和两个时间片(近期:2041-2060 年和远期:2081-2100 年)。紫外线辐射率预测显示,远期夏半球的紫外线辐射率会发生明显变化。南半球中高纬度地区总有机碳的增加导致夏至紫外线辐射率下降。然而,预测结果并没有表明南美洲、澳大利亚和南部非洲的曝晒条件是安全的。相反,在整个本世纪,太阳正午前后 10 至 20 分钟的曝晒仍足以诱发 III 型皮肤的人出现红斑。在阿根廷南部和智利,本世纪冬至日正午的紫外线辐射对 III 型皮肤合成维生素 D 的不足量保持不变。在北半球,人口稠密地区夏至日的紫外线辐射指数和紫外线吸收率应保持在较高水平(紫外线辐射指数≥8;紫外线吸收率约为 7.0 kJ m-2)。在北纬 45°以上,紫外线辐射水平不足以在北方冬季在 III 型皮肤中合成维生素 D。我们的研究结果表明,气候变化将通过太阳紫外线辐射过量或不足影响人类健康。
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来源期刊
Photochemical & Photobiological Sciences
Photochemical & Photobiological Sciences 生物-生化与分子生物学
CiteScore
5.60
自引率
6.50%
发文量
201
审稿时长
2.3 months
期刊介绍: A society-owned journal publishing high quality research on all aspects of photochemistry and photobiology.
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