Two-dimensional Sb net generated nontrivial topological states in SmAgSb2 probed by quantum oscillations

Jian Yuan, Xian-Biao Shi, Hong Du, Tian Li, Chuanying Xi, Xia Wang, Wei Xia, Bao-Tian Wang, Ruidan Zhong, Yan-Feng Guo
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Abstract

The REAgSb2 (RE = rare earth and Y) family has drawn considerable research interest because the two-dimensional Sb net in their crystal structure hosts topological fermions and hence rich topological properties. We report herein the magnetization and magnetotransport measurements of SmAgSb2 single crystal, which unveil very large magnetoresistance and high carrier mobility up to 6.2×103% and 5.58×103 cm2V-1s-1, respectively. The analysis of both Shubnikov-de Haas and de Haas-van Alphen quantum oscillations indicates nontrivial Berry phases in the paramagnetic state while trivial Berry curvature in the antiferromagnetic state, indicating a topological phase transition induced by the antiferromagnetic order. It is also supported by the first-principles calculations. The results not only provide a new interesting topological material but also offer valuable insights into the correlation between magnetism and nontrivial topological states.
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通过量子振荡探测 SmAgSb2 中二维 Sb 网产生的非难拓扑态
REAgSb2(RE = 稀土和 Y)家族引起了人们相当大的研究兴趣,因为其晶体结构中的二维 Sb 网承载着拓扑费米子,因而具有丰富的拓扑特性。我们在此报告了 SmAgSb2 单晶的磁化和磁迁移测量结果,结果显示其磁电阻和载流子迁移率分别高达 6.2×103% 和 5.58×103 cm2V-1s-1。对舒布尼科夫-德哈斯量子振荡和德哈斯-范阿尔芬量子振荡的分析表明,顺磁态存在非三相贝里相,而反铁磁态存在三相贝里曲率,这表明反铁磁秩序诱导了拓扑相变。这也得到了第一原理计算的支持。这些结果不仅提供了一种新的有趣的拓扑材料,而且为研究磁性与非三重拓扑态之间的相关性提供了宝贵的见解。
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