Low frequency signal detection via correlated Ramsey measurements

IF 2 3区 化学 Q3 BIOCHEMICAL RESEARCH METHODS Journal of magnetic resonance Pub Date : 2024-05-07 DOI:10.1016/j.jmr.2024.107691
Santiago Oviedo-Casado , Javier Prior , Javier Cerrillo
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Abstract

The low frequency region of the spectrum is a challenging regime for quantum probes. We support the idea that, in this regime, performing Ramsey measurements carefully controlling the time at which each measurement is initiated is an excellent signal detection strategy. We use the Fisher information to demonstrate a high quality performance in the low frequency regime, compared to more elaborated measurement sequences, and to optimize the correlated Ramsey sequence according to any given experimental parameters, showing that correlated Ramsey rivals with state-of-the-art protocols, and can even outperform commonly employed sequences such as dynamical decoupling in the detection of low frequency signals. Contrary to typical quantum detection protocols for oscillating signals, which require adjusting the time separation between pulses to match the half period of the target signal, and consequently see their scope limited to signals whose period is shorter than the characteristic decoherence time of the probe, or to those protocols whose target is primarily static signals, the time-tagged correlated Ramsey sequence simultaneously tracks the amplitude and the phase information of the target signal, regardless of its frequency, which crucially permits correlating measurements in post-processing, leading to efficient spectral reconstruction.

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通过相关拉姆齐测量进行低频信号检测
对于量子探测器来说,频谱的低频区是一个具有挑战性的系统。我们支持这样一种观点,即在这种情况下,仔细控制每次测量开始的时间进行拉姆齐测量是一种极佳的信号探测策略。我们利用费雪信息证明了与更复杂的测量序列相比,相关拉姆齐序列在低频系统中的高质量性能,并根据任何给定的实验参数对相关拉姆齐序列进行了优化,表明相关拉姆齐可与最先进的协议相媲美,甚至在低频信号探测中优于动态解耦等常用序列。典型的振荡信号量子探测协议需要调整脉冲之间的时间间隔以匹配目标信号的半周期,因此其探测范围仅限于周期短于探针特征退相干时间的信号,或者那些以静态信号为主要目标的协议,与之相反,时间标记的相关拉姆齐序列可同时跟踪目标信号的振幅和相位信息(无论其频率如何),这使得后处理中的相关测量成为可能,从而实现高效的频谱重构。
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来源期刊
CiteScore
3.80
自引率
13.60%
发文量
150
审稿时长
69 days
期刊介绍: The Journal of Magnetic Resonance presents original technical and scientific papers in all aspects of magnetic resonance, including nuclear magnetic resonance spectroscopy (NMR) of solids and liquids, electron spin/paramagnetic resonance (EPR), in vivo magnetic resonance imaging (MRI) and spectroscopy (MRS), nuclear quadrupole resonance (NQR) and magnetic resonance phenomena at nearly zero fields or in combination with optics. The Journal''s main aims include deepening the physical principles underlying all these spectroscopies, publishing significant theoretical and experimental results leading to spectral and spatial progress in these areas, and opening new MR-based applications in chemistry, biology and medicine. The Journal also seeks descriptions of novel apparatuses, new experimental protocols, and new procedures of data analysis and interpretation - including computational and quantum-mechanical methods - capable of advancing MR spectroscopy and imaging.
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