Lattice-commensurate skyrmion texture in a centrosymmetric breathing kagome magnet

IF 5.4 1区 物理与天体物理 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY npj Quantum Materials Pub Date : 2024-05-23 DOI:10.1038/s41535-024-00654-2
Max Hirschberger, Bertalan G. Szigeti, Mamoun Hemmida, Moritz M. Hirschmann, Sebastian Esser, Hiroyuki Ohsumi, Yoshikazu Tanaka, Leonie Spitz, Shang Gao, Kamil K. Kolincio, Hajime Sagayama, Hironori Nakao, Yuichi Yamasaki, László Forró, Hans-Albrecht Krug von Nidda, Istvan Kezsmarki, Taka-hisa Arima, Yoshinori Tokura
{"title":"Lattice-commensurate skyrmion texture in a centrosymmetric breathing kagome magnet","authors":"Max Hirschberger, Bertalan G. Szigeti, Mamoun Hemmida, Moritz M. Hirschmann, Sebastian Esser, Hiroyuki Ohsumi, Yoshikazu Tanaka, Leonie Spitz, Shang Gao, Kamil K. Kolincio, Hajime Sagayama, Hironori Nakao, Yuichi Yamasaki, László Forró, Hans-Albrecht Krug von Nidda, Istvan Kezsmarki, Taka-hisa Arima, Yoshinori Tokura","doi":"10.1038/s41535-024-00654-2","DOIUrl":null,"url":null,"abstract":"<p>Skyrmion lattices (SkL) in centrosymmetric materials typically have a magnetic period on the nanometer-scale, so that the coupling between magnetic superstructures and the underlying crystal lattice cannot be neglected. We reveal the commensurate locking of a SkL to the atomic lattice in Gd<sub>3</sub>Ru<sub>4</sub>Al<sub>12</sub> via high-resolution resonant elastic x-ray scattering (REXS). Weak easy-plane magnetic anisotropy, demonstrated here by a combination of ferromagnetic resonance and REXS, penalizes placing a skyrmion core on a site of the atomic lattice. Under these conditions, a commensurate SkL, locked to the crystal lattice, is stable at finite temperatures – but gives way to a competing incommensurate ground state upon cooling. We discuss the role of Umklapp-terms in the Hamiltonian for the formation of this lattice-locked state, its magnetic space group, and the role of slight discommensurations, or (line) defects in the magnetic texture. We also contrast our findings with the case of SkLs in noncentrosymmetric material platforms.</p>","PeriodicalId":19283,"journal":{"name":"npj Quantum Materials","volume":"75 1","pages":""},"PeriodicalIF":5.4000,"publicationDate":"2024-05-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"npj Quantum Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1038/s41535-024-00654-2","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Skyrmion lattices (SkL) in centrosymmetric materials typically have a magnetic period on the nanometer-scale, so that the coupling between magnetic superstructures and the underlying crystal lattice cannot be neglected. We reveal the commensurate locking of a SkL to the atomic lattice in Gd3Ru4Al12 via high-resolution resonant elastic x-ray scattering (REXS). Weak easy-plane magnetic anisotropy, demonstrated here by a combination of ferromagnetic resonance and REXS, penalizes placing a skyrmion core on a site of the atomic lattice. Under these conditions, a commensurate SkL, locked to the crystal lattice, is stable at finite temperatures – but gives way to a competing incommensurate ground state upon cooling. We discuss the role of Umklapp-terms in the Hamiltonian for the formation of this lattice-locked state, its magnetic space group, and the role of slight discommensurations, or (line) defects in the magnetic texture. We also contrast our findings with the case of SkLs in noncentrosymmetric material platforms.

Abstract Image

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
中心对称呼吸式卡戈米磁体中与晶格相称的天磁纹理
中心对称材料中的Skyrmion晶格(SkL)通常具有纳米级的磁周期,因此磁性超结构与底层晶格之间的耦合不容忽视。我们通过高分辨率共振弹性 X 射线散射(REXS)揭示了 Gd3Ru4Al12 中 SkL 与原子晶格的相称锁定。这里通过铁磁共振和 REXS 的结合证明了弱易平面磁各向异性,这不利于将一个锡基磁核放置在原子晶格的一个位置上。在这些条件下,锁定在晶格上的同位SkL在有限温度下是稳定的--但冷却后会让位于竞争性的非同位基态。我们讨论了这种晶格锁定态形成的哈密顿方程中 Umklapp 子的作用、其磁性空间群以及磁性纹理中轻微不相称或(线)缺陷的作用。我们还将研究结果与非中心对称材料平台中的 SkLs 情况进行了对比。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 去求助
来源期刊
npj Quantum Materials
npj Quantum Materials Materials Science-Electronic, Optical and Magnetic Materials
CiteScore
10.60
自引率
3.50%
发文量
107
审稿时长
6 weeks
期刊介绍: npj Quantum Materials is an open access journal that publishes works that significantly advance the understanding of quantum materials, including their fundamental properties, fabrication and applications.
期刊最新文献
Spin-orbit entangled moments and magnetic exchange interactions in cobalt-based honeycomb magnets BaCo2(XO4)2 (X = P, As, Sb) Intrinsic second-order topological insulators in two-dimensional polymorphic graphyne with sublattice approximation Quantum phase transition and composite excitations of antiferromagnetic spin trimer chains in a magnetic field 3D Heisenberg universality in the van der Waals antiferromagnet NiPS3 Multinode quantum spin liquids in extended Kitaev honeycomb models
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1