Heterostructured Ti3C2Tx/carbon nanohorn-based gas sensor for NH3 detection at room temperature

Abstract

In this study, a two-dimensional Ti3C2Tx MXene compounded with carbon nanohorn (CNH) by an electrostatic self-assembly method was proposed and then fabricated as room temperature ammonia (NH3) gas sensors. The successful preparation of the Ti3C2Tx/CNH nanocomposite has been characterized in detail. The NH3 sensing performance based on Ti3C2Tx/CNH also has been tested at room temperature. The optimal Ti3C2Tx/CNH sensor has a response value of 21.6% to 100 ppm NH3 at room temperature, which is 10 times higher than that of the pure Ti3C2Tx sensor. Furthermore, this sensor is endowed with excellent selectivity, reliable long-term stability, and reproducibility. The enhanced sensing performance is associated with the interconnected structure and the synergistic effect of Ti3C2Tx and CNH. This work provides an effective way to prepare MXene-based sensitive materials for NH3 sensors, which shows excellent NH3 detection potential at room temperature.