CFD-PBM simulation of power law fluid in a bubble column reactor

IF 17.7 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-06-17 DOI:10.1515/ijcre-2024-0010
Mengqiang Duan, Shao-Bai Li, Manju L. Bhusal, Wei Zhang, Yuhuan Ding
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Abstract

Abstract A computational fluid dynamics coupled population balance model (CFD-PBM) was used to numerically simulate the fluid dynamics of bubble swarms in a bubble column containing non-Newtonian fluids. The effects of superficial gas velocity (U g ), the consistency index (K), and the flow index (n) on bubble size distribution (BSD), gas holdup, and fluid dynamic viscosity in a bubble column were analyzed at both local and overall scales. As U g increases, the bubble breakup occurs excessively, the gas holdup increases, and the dynamic viscosity decreases. K and n were used to characterize the rheological properties of power law fluid. As K increases, fluid viscosity increases, bubble breakup rate decreases, gas holdup in the top zone is slightly lower than in the middle zone, and dynamic viscosity increases. Within the range of n from 0.45 to 1.07, when n is smallest, the relative frequency of bubbles smaller than the initial size is relatively large, and the overall and local gas holdup are the highest. When n = 1.07, the fluid exhibits shear-thickening properties, and the dynamic viscosity variations are significant.
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气泡塔反应器中幂律流体的 CFD-PBM 模拟
摘要 采用计算流体动力学耦合种群平衡模型(CFD-PBM)对含有非牛顿流体的气泡柱中气泡群的流体动力学进行了数值模拟。从局部和整体尺度分析了表层气体速度(U g)、稠度指数(K)和流动指数(n)对气泡柱中气泡大小分布(BSD)、气体滞留和流体动态粘度的影响。随着 U g 的增大,气泡破裂过度,气体滞留增加,动态粘度降低。K 和 n 用于描述幂律流体的流变特性。随着 K 的增大,流体粘度增大,气泡破裂率降低,顶部区域的气体滞留略低于中间区域,动态粘度增大。在 n 从 0.45 到 1.07 的范围内,当 n 最小时,小于初始尺寸的气泡的相对频率相对较大,整体和局部气体截留率最高。当 n = 1.07 时,流体表现出剪切增稠特性,动态粘度变化显著。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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