Synthesis, Characterization, and OFET Characteristics of p-Type Organic Semiconductors Incorporating Diketopyrrolopyrrole and Thiadiazole-Quinoxaline Acceptors

IF 16.4 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-06-13 DOI:10.1093/chemle/upae115

Naohiro Takahashi, Tomoki Nishiyama, Weichun Weng, Yuki Miwa, Shinsuke Marumoto, Hirotaka Kitoh-Nishioka, Senku Tanaka, Takashi Okubo

引用次数: 0

Abstract

P-type Organic Semiconductors, TQx5-BT-DPP8 (1a) and TQx5-BT-DPP20 (1b), consisting of a donor unit of bithiophene (BT) and two acceptor units of thiadiazole quinoxaline (TQx) and diketopyrrolopyrrole (DPP), were synthesized, and their electronic states and physical properties were elucidated. These semiconductors demonstrate strong absorption extending from the visible to the near-infrared region, functioning effectively as strong donor dyes. The organic field-effect transistors (OFETs) exhibited normally on transistor characteristics, with carrier mobilities of 1.1×10−3 cm2/Vs for 1a and 3.3×10−4 cm2/Vs for 1b.

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包含二酮吡咯并噻二唑-喹喔啉受体的 p 型有机半导体的合成、表征和 OFET 特性

合成了 P 型有机半导体 TQx5-BT-DPP8 (1a) 和 TQx5-BT-DPP20 (1b)，它们由一个供体单元噻吩（BT）和两个受体单元噻二唑喹喔啉（TQx）和二酮吡咯（DPP）组成，并阐明了它们的电子状态和物理性质。这些半导体显示出从可见光到近红外区域的强烈吸收，可有效地用作强供体染料。有机场效应晶体管（OFET）显示出正常的晶体管特性，1a 和 1b 的载流子迁移率分别为 1.1×10-3 cm2/Vs和 3.3×10-4 cm2/Vs。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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来源期刊

Accounts of Chemical Research 化学-化学综合

CiteScore

31.40

自引率

1.10%

发文量

312

审稿时长

2 months

期刊介绍： Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.

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