Mechanochemical and Sonochemical Obtaining of Nanosized Oxides Materials and Catalysts: A Review

IF 0.7 4区 化学 Q4 CHEMISTRY, MULTIDISCIPLINARY Theoretical and Experimental Chemistry Pub Date : 2024-06-06 DOI:10.1007/s11237-024-09797-6
V. O. Zazhigalov, O. V. Sachuk, O. V. Kiziun, O. A. Diyuk, I. V. Bacherikova
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Abstract

The promising application of mechanochemical (MC) and sonochemical (SC) synthesis methods for the obtaining of nano-dispersed oxide materials with a perovskite structure (BaTiO3, CaTiO3, and LiNbO3) and higher specific surface value as compared to samples obtained by traditional methods is shown. Synthesized samples exhibit high photocatalytic activity in the oxidative degradation of metronidazole and chloramphenicol drugs, as well as a promethrin herbicide in an aqueous medium exceeding known analogs. The possibilities of MC and SC in the synthesis of zinc and bismuth molybdates with the obtaining of their nanostructures with different morphologies, in particular bars, needles, rods, and spheres, are shown. It is established that prepared samples demonstrate high activity in the processes of ethanol oxidation to acetaldehyde (β-ZnMoO4) or acetic acid (α-ZnMoO4), oxidative dehydrogenation of hydrocarbons of the industrial fraction of oil processing with the obtaining of 1,3-butadiene (Bi2Mo3O12).

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纳米氧化物材料和催化剂的机械化学和声化学制备:综述
在获得具有包晶结构的纳米分散氧化物材料(BaTiO3、CaTiO3 和 LiNbO3)时,机械化学(MC)和声化学(SC)合成方法的应用前景广阔,与传统方法获得的样品相比,其比表面积更高。合成的样品在水介质中氧化降解甲硝唑和氯霉素药物以及除草剂丙炔菊酯时表现出的光催化活性超过了已知的类似物。MC 和 SC 在合成钼酸锌和钼酸铋时,可获得不同形态的纳米结构,特别是条状、针状、棒状和球状结构。实验证明,制备的样品在乙醇氧化成乙醛(β-ZnMoO4)或乙酸(α-ZnMoO4)、石油加工工业馏分中的碳氢化合物氧化脱氢生成 1,3-丁二烯(Bi2Mo3O12)的过程中表现出很高的活性。
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来源期刊
Theoretical and Experimental Chemistry
Theoretical and Experimental Chemistry CHEMISTRY, MULTIDISCIPLINARY-
CiteScore
1.60
自引率
10.00%
发文量
30
审稿时长
6-12 weeks
期刊介绍: Theoretical and Experimental Chemistry is a journal for the rapid publication of research communications and reviews on modern problems of physical chemistry such as: a) physicochemical bases, principles, and methods for creation of novel processes, compounds, and materials; b) physicochemical principles of chemical process control, influence of external physical forces on chemical reactions; c) physical nanochemistry, nanostructures and nanomaterials, functional nanomaterials, size-dependent properties of materials.
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