Interface-Suppressed Nematicity and Enhanced Superconducting Pairing Strength of FeSe/NdFeO3 in the Low-Doping Regime

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2024-06-27 DOI:10.1021/acs.nanolett.4c01493
Chihao Li, Yuanhe Song, Xiaoxiao Wang, Minyinan Lei, Xiaoyang Chen, Haichao Xu*, Rui Peng* and Donglai Feng*, 
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Abstract

The discovery of interfacial superconductivity in monolayer FeSe/oxides has spurred intensive research interest. Here we not only extend the FeSe/FeOx superconducting interface to FeSe/NdFeO3 but also establish robust interface-enhanced superconductivity at a very low doping level. Specifically, well-annealed FeSe/NdFeO3 exhibits a low doping level of 0.038–0.046 e/Fe with a larger superconducting pairing gap without a nematic gap, indicating an enhancement of the enhanced superconducting pairing strength and suppression of nematicity by the FeSe/FeOx interface compared with those of thick FeSe films. These results improve our understanding of the roles of the oxide interface in the low-electron-doped regime.

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FeSe/NdFeO3在低掺杂状态下的界面抑制向列性和增强超导配对强度
单层 FeSe/氧化物界面超导性的发现激发了人们浓厚的研究兴趣。在这里,我们不仅将 FeSe/FeOx 超导界面扩展到了 FeSe/NdFeO3,而且还在极低的掺杂水平下建立了稳健的界面增强超导性。具体来说,退火良好的 FeSe/NdFeO3 在 0.038-0.046 e-/Fe 的低掺杂水平下具有更大的超导配对间隙,而不存在向列间隙,这表明与厚 FeSe 薄膜相比,FeSe/FeOx 界面增强了超导配对强度并抑制了向列性。这些结果加深了我们对氧化物界面在低电子掺杂体系中的作用的理解。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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