Design of a Compact Multicyclic High-Performance Atmospheric Water Harvester for Arid Environments

IF 19.3 1区 材料科学 Q1 CHEMISTRY, PHYSICAL ACS Energy Letters Pub Date : 2024-06-26 DOI:10.1021/acsenergylett.4c01061
Xiangyu Li*, Bachir El Fil*, Buxuan Li, Gustav Graeber, Adela C. Li, Yang Zhong, Mohammed Alshrah, Chad T. Wilson and Emily Lin, 
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Abstract

Water scarcity remains a grand challenge across the globe. Sorption-based atmospheric water harvesting (SAWH) is an emerging and promising solution for water scarcity, especially in arid and noncoastal regions. Traditional approaches to AWH such as fog harvesting and dewing are often not applicable in an arid environment (<30% relative humidity (RH)), whereas SAWH has demonstrated great potential to provide fresh water under a wide range of climate conditions. Despite advances in materials development, most demonstrated SAWH devices still lack sufficient water production. In this work, we focus on the adsorption bed design to achieve high water production, multicyclic operation, and a compact form factor (high material loading per heat source contact area). The modeling efforts and experimental validation illustrate an optimized design space with a fin-array adsorption bed enabled by high-density waste heat, which promises 5.826 Lwater kgsorbent–1 day–1 at 30% RH within a compact 1 L adsorbent bed and commercial adsorbent materials.

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为干旱环境设计紧凑型多循环高性能大气采水器
水资源短缺仍然是全球面临的巨大挑战。基于吸附作用的大气集水(SAWH)是解决水资源短缺问题的一种新兴且前景广阔的方法,尤其是在干旱和非沿海地区。传统的大气集水方法,如雾收集和脱水,往往不适用于干旱环境(相对湿度为 30%),而吸附式大气集水已证明具有在各种气候条件下提供淡水的巨大潜力。尽管在材料开发方面取得了进展,但大多数已展示的 SAWH 设备仍然缺乏足够的产水量。在这项工作中,我们将重点放在吸附床的设计上,以实现高产水、多循环运行和紧凑的外形尺寸(单位热源接触面积的高材料负荷)。建模工作和实验验证说明了利用高密度余热的鳍阵吸附床的优化设计空间,在 30% 相对湿度条件下,使用 1 L 紧凑型吸附床和商用吸附材料,可实现 5.826 Lwater kgsorbent-1 day-1。
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来源期刊
ACS Energy Letters
ACS Energy Letters Energy-Renewable Energy, Sustainability and the Environment
CiteScore
31.20
自引率
5.00%
发文量
469
审稿时长
1 months
期刊介绍: ACS Energy Letters is a monthly journal that publishes papers reporting new scientific advances in energy research. The journal focuses on topics that are of interest to scientists working in the fundamental and applied sciences. Rapid publication is a central criterion for acceptance, and the journal is known for its quick publication times, with an average of 4-6 weeks from submission to web publication in As Soon As Publishable format. ACS Energy Letters is ranked as the number one journal in the Web of Science Electrochemistry category. It also ranks within the top 10 journals for Physical Chemistry, Energy & Fuels, and Nanoscience & Nanotechnology. The journal offers several types of articles, including Letters, Energy Express, Perspectives, Reviews, Editorials, Viewpoints and Energy Focus. Additionally, authors have the option to submit videos that summarize or support the information presented in a Perspective or Review article, which can be highlighted on the journal's website. ACS Energy Letters is abstracted and indexed in Chemical Abstracts Service/SciFinder, EBSCO-summon, PubMed, Web of Science, Scopus and Portico.
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