Transfer of hexagonal boron nitride quantum emitters onto arbitrary substrates with zero thermal budget

IF 5.3 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY APL Materials Pub Date : 2024-07-02 DOI:10.1063/5.0218367
Dante J. O’Hara, Hsun-Jen Chuang, Kathleen M. McCreary, Mehmet A. Noyan, Sung-Joon Lee, Enrique D. Cobas, Berend T. Jonker
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Abstract

The van der Waals material hexagonal boron nitride (hBN) has emerged as a promising candidate for hosting room temperature single-photon emitters (SPEs) for next-generation quantum technologies. However, the requirement of a high temperature anneal (850 °C or higher) to activate the SPEs in hBN makes it difficult to integrate into hybrid structures that cannot tolerate such temperatures, including all silicon-based circuits. In this work, we present a method to deterministically activate quantum emitters in multilayered hBN on a process substrate, followed by a zero thermal budget transfer to a target substrate. This technique does not lead to any degradation or loss of photon purity in the hBN emitters and provides a procedure for combining high-purity emitters with other exciting photonic, magnetic, or electrical properties to explore new physical phenomena. The ability to transfer hBN emitters onto arbitrary substrates creates new technological possibilities to incorporate these quantum photonic properties into photonic integrated circuits and plasmonic devices.
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将六方氮化硼量子发射器转移到零热预算的任意基底上
范德瓦耳斯材料六方氮化硼(hBN)已成为承载室温单光子发射器(SPE)的理想候选材料,可用于下一代量子技术。然而,由于需要高温退火(850 ℃ 或更高)才能激活氮化硼中的单光子发射器,因此很难将其集成到无法耐受这种温度的混合结构中,包括所有硅基电路。在这项工作中,我们提出了一种方法,可在工艺基底上确定性地激活多层氢化硼中的量子发射器,然后将零热预算转移到目标基底上。这种技术不会导致 hBN 发射器中的光子纯度发生任何退化或损失,并提供了一种将高纯度发射器与其他令人兴奋的光子、磁性或电学特性相结合的程序,以探索新的物理现象。将 hBN 发射器转移到任意基底上的能力为将这些量子光子特性融入光子集成电路和等离子器件创造了新的技术可能性。
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来源期刊
APL Materials
APL Materials NANOSCIENCE & NANOTECHNOLOGYMATERIALS SCIE-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
9.60
自引率
3.30%
发文量
199
审稿时长
2 months
期刊介绍: APL Materials features original, experimental research on significant topical issues within the field of materials science. In order to highlight research at the forefront of materials science, emphasis is given to the quality and timeliness of the work. The journal considers theory or calculation when the work is particularly timely and relevant to applications. In addition to regular articles, the journal also publishes Special Topics, which report on cutting-edge areas in materials science, such as Perovskite Solar Cells, 2D Materials, and Beyond Lithium Ion Batteries.
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