MoS2@CoFe-MOF catalysts by one-pot hydrothermal synthesis enhanced electron interaction between MoS2 nanoflower and bimetallic MOF for efficient oxygen evolution

IF 2.7 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY New Journal of Chemistry Pub Date : 2024-07-10 DOI:10.1039/d4nj02380c
Jiahui Li, Yufen Wang, Qinyuan Yu, Xuedong Wei
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引用次数: 0

Abstract

A kind of MoS2@CoFe-MOF electrocatalyst was prepared on carbon cloth by one-pot hydrothermal method. The excellent electrocatalysts activity of MoS2@CoFe-MOF are demonstrated. It can use the overpotential of 220 mV and 405 mV respectively to drive 10 mA cm-2 and 50 mA cm-2. It is indicated that the MoS2@CoFe-MOF electrode exhibits excellent stability at the end of 48000 s, and it has the highest electrochemical activity specific surface area and the lowest charge transfer resistance. This work proposes a promising approach for hydrogen production by electrolysis of water using electrocatalysts composed of non precious transition metal sulfides and bimetallic MOFs in energy chemistry.
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通过一锅水热法合成 MoS2@CoFe-MOF 催化剂,增强 MoS2 纳米花与双金属 MOF 之间的电子相互作用,实现高效氧进化
采用一锅水热法在碳布上制备了一种MoS2@CoFe-MOF电催化剂。结果表明,MoS2@CoFe-MOF 具有优异的电催化活性。它能分别用 220 mV 和 405 mV 的过电位驱动 10 mA cm-2 和 50 mA cm-2。结果表明,MoS2@CoFe-MOF 电极在 48000 秒结束时表现出极佳的稳定性,并且具有最高的电化学活性比表面积和最低的电荷转移电阻。这项研究为能源化学领域利用非贵重过渡金属硫化物和双金属 MOF 组成的电催化剂电解水制氢提出了一种可行的方法。
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来源期刊
New Journal of Chemistry
New Journal of Chemistry 化学-化学综合
CiteScore
5.30
自引率
6.10%
发文量
1832
审稿时长
2 months
期刊介绍: A journal for new directions in chemistry
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