{"title":"Design principle of anti‐corrosive photocatalyst for large‐scale hydrogen production","authors":"Spandana Gonuguntla, Bhavya Jaksani, Aparna Jamma, Chandra Shobha Vennapoosa, Debabrata Chatterjee, Ujjwal Pal","doi":"10.1002/wene.530","DOIUrl":null,"url":null,"abstract":"With the most advances made so far in terms of photocatalyst design and preparation (inorganic photoredox nanoparticles), researchers of different expertise joined together to address sustainable energy conversion. Despite notable advancements in creating exceptionally active photocatalysts, the practical scalability of these innovations is hindered by issues such as ineffective utilization of solar energy and mass transport, recombination reactions, catalyst instability, and photo corrosion of the catalyst. In this roadmap review, we brief the fundamentals, latest progress, outstanding challenges, and novel design methodology for anticorrosive photocatalysts favorable to large‐scale hydrogen production. To enable the effective scaling of photocatalysis, beyond the inherent activity of photocatalysts, a range of additional factors are considered, with a primary focus on the design of photocatalytic systems. This review underlines the significance of well‐structured photocatalyst design and evaluation for achieving reproducibility and using dependable research methodology for conducting rigorous experiments. The recommendations are directed at reducing the uncertainty surrounding the optimism presented in published research, and we spotlight our recent research advancements. Importantly, the synergistic integration of design principles and research methodologies to enhance the anti‐corrosion properties of photocatalysts may pave the way for a practical technology to utilize solar energy for large‐scale hydrogen production efficiently.This article is categorized under:<jats:list list-type=\"simple\"> <jats:list-item>Sustainable Energy > Solar Energy</jats:list-item> </jats:list>","PeriodicalId":48766,"journal":{"name":"Wiley Interdisciplinary Reviews-Energy and Environment","volume":"39 1","pages":""},"PeriodicalIF":5.4000,"publicationDate":"2024-07-12","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Wiley Interdisciplinary Reviews-Energy and Environment","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1002/wene.530","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
引用次数: 0
Abstract
With the most advances made so far in terms of photocatalyst design and preparation (inorganic photoredox nanoparticles), researchers of different expertise joined together to address sustainable energy conversion. Despite notable advancements in creating exceptionally active photocatalysts, the practical scalability of these innovations is hindered by issues such as ineffective utilization of solar energy and mass transport, recombination reactions, catalyst instability, and photo corrosion of the catalyst. In this roadmap review, we brief the fundamentals, latest progress, outstanding challenges, and novel design methodology for anticorrosive photocatalysts favorable to large‐scale hydrogen production. To enable the effective scaling of photocatalysis, beyond the inherent activity of photocatalysts, a range of additional factors are considered, with a primary focus on the design of photocatalytic systems. This review underlines the significance of well‐structured photocatalyst design and evaluation for achieving reproducibility and using dependable research methodology for conducting rigorous experiments. The recommendations are directed at reducing the uncertainty surrounding the optimism presented in published research, and we spotlight our recent research advancements. Importantly, the synergistic integration of design principles and research methodologies to enhance the anti‐corrosion properties of photocatalysts may pave the way for a practical technology to utilize solar energy for large‐scale hydrogen production efficiently.This article is categorized under:Sustainable Energy > Solar Energy
期刊介绍:
Wiley Interdisciplinary Reviews: Energy and Environmentis a new type of review journal covering all aspects of energy technology, security and environmental impact.
Energy is one of the most critical resources for the welfare and prosperity of society. It also causes adverse environmental and societal effects, notably climate change which is the severest global problem in the modern age. Finding satisfactory solutions to the challenges ahead will need a linking of energy technology innovations, security, energy poverty, and environmental and climate impacts. The broad scope of energy issues demands collaboration between different disciplines of science and technology, and strong interaction between engineering, physical and life scientists, economists, sociologists and policy-makers.