Quantized Microcavity Polariton Lasing Based on InGaN Localized Excitons

Nanomaterials Pub Date : 2024-07-14 DOI:10.3390/nano14141197
Huying Zheng, Runchen Wang, Xuebing Gong, Junxing Dong, Lisheng Wang, Jingzhuo Wang, Yifan Zhang, Yan Shen, Huanjun Chen, Baijun Zhang, Hai Zhu
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Abstract

Exciton–polaritons, which are bosonic quasiparticles with an extremely low mass, play a key role in understanding macroscopic quantum effects related to Bose–Einstein condensation (BEC) in solid-state systems. The study of trapped polaritons in a potential well provides an ideal platform for manipulating polariton condensates, enabling polariton lasing with specific formation in k-space. Here, we realize quantized microcavity polariton lasing in simple harmonic oscillator (SHO) states based on spatial localized excitons in InGaN/GaN quantum wells (QWs). Benefiting from the high exciton binding energy (90 meV) and large oscillator strength of the localized exciton, room-temperature (RT) polaritons with large Rabi splitting (61 meV) are obtained in a strongly coupled microcavity. The manipulation of polariton condensates is performed through a parabolic potential well created by optical pump control. Under the confinement situation, trapped polaritons are controlled to be distributed in the selected quantized energy sublevels of the SHO state. The maximum energy spacing of 11.3 meV is observed in the SHO sublevels, indicating the robust polariton trapping of the parabolic potential well. Coherent quantized polariton lasing is achieved in the ground state of the SHO state and the coherence property of the lasing is analyzed through the measurements of spatial interference patterns and g(2)(τ). Our results offer a feasible route to explore the manipulation of macroscopic quantum coherent states and to fabricate novel polariton devices towards room-temperature operations.
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基于 InGaN 局域激子的量化微腔极化子激光技术
激子-极化子是质量极低的玻色性准粒子,在理解固态系统中与玻色-爱因斯坦凝聚(BEC)有关的宏观量子效应方面发挥着关键作用。研究被困在势阱中的极化子为操纵极化子凝聚物提供了一个理想的平台,从而可以在 k 空间中形成特定的极化子激光。在这里,我们基于 InGaN/GaN 量子阱(QWs)中的空间局域激子,在简谐振荡器(SHO)态中实现了量子化微腔极化子激光。利用高激子结合能(90 meV)和局部激子的大振荡器强度,在强耦合微腔中获得了具有大拉比分裂(61 meV)的室温(RT)极化子。对极化子凝聚态的操纵是通过光泵控制产生的抛物线势阱来实现的。在约束条件下,被捕获的极化子被控制分布在 SHO 状态的选定量子化能级中。在 SHO 子级中观察到的最大能距为 11.3 meV,表明抛物势阱具有强大的极化子捕获能力。在 SHO 状态的基态中实现了相干量子化极化子激光,并通过测量空间干涉模式和 g(2)(τ)分析了激光的相干特性。我们的研究结果为探索操纵宏观量子相干态和制造新型极化子器件以实现室温操作提供了一条可行的途径。
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