Enhanced Efficient Solar Evaporation of Co/CoO Loaded on the Tobacco Stem Under Visible Light

IF 6.5 3区 材料科学 Q2 GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY Advanced Sustainable Systems Pub Date : 2024-07-26 DOI:10.1002/adsu.202400349
Yu Liu, Chunyan Zhang, Anlong Zhang, Jindi Zhang, Lili Zhang, Mengyang Huang, Jiaqiang Wang
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Abstract

Solar-driven water evaporation is an emerging technology in green technology of seawater desalination and sewage treatment. However, the quality of high cost, complex manufacturing, and a small amount of synthetic materials is the main obstacle to large-scale applications. Biological carbon-based materials have a large and efficient heat exchange area due to the naturally abundant pore structure, which plays an important role in regulating convection and radiant heat loss. However, single-component carbon materials have limited photothermal conversion performance, which limits their large-scale application. In this work, tobacco stem (TS) organisms loaded with Co/CoO nanoparticles are successfully prepared by one-step pyrolysis. The synergistic effect of Co/CoO nanostructures and biocarbon materials enhances water evaporation performance, widening the absorption range of the material across the entire solar spectrum, and expanding the range of energy that can be converted into heat. Specifically, the water evaporation rate and photothermal conversion efficiency of TS -Co/CoO (0.20) reached 2.22 kg m−2 h−1 and 139.4%, respectively, and its evaporation rate is 1.7 times the direct carbonized tobacco and 4.35 times the pure water. This work provides a research idea for the multifunctional and effective utilization of waste biomass materials and the construction of bionic structure solar photothermal materials.

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在可见光下提高烟草茎秆上负载的 Co/CoO 的太阳能蒸发效率
太阳能驱动水蒸发是海水淡化和污水处理绿色技术中的一项新兴技术。然而,成本高、制造复杂、合成材料量少等质量问题是大规模应用的主要障碍。生物碳基材料因天然丰富的孔隙结构而具有较大且高效的热交换面积,在调节对流和辐射热损失方面发挥着重要作用。然而,单组分碳材料的光热转换性能有限,限制了其大规模应用。本研究通过一步热解法成功制备了负载 Co/CoO 纳米颗粒的烟草茎(TS)生物体。Co/CoO 纳米结构与生物碳材料的协同效应增强了水蒸发性能,拓宽了材料在整个太阳光谱中的吸收范围,扩大了可转化为热能的能量范围。具体来说,TS -Co/CoO (0.20) 的水蒸发率和光热转换效率分别达到了 2.22 kg m-2 h-1 和 139.4%,其蒸发率是直接碳化烟草的 1.7 倍和纯水的 4.35 倍。这项工作为废弃生物质材料的多功能有效利用和仿生结构太阳能光热材料的构建提供了研究思路。
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来源期刊
Advanced Sustainable Systems
Advanced Sustainable Systems Environmental Science-General Environmental Science
CiteScore
10.80
自引率
4.20%
发文量
186
期刊介绍: Advanced Sustainable Systems, a part of the esteemed Advanced portfolio, serves as an interdisciplinary sustainability science journal. It focuses on impactful research in the advancement of sustainable, efficient, and less wasteful systems and technologies. Aligned with the UN's Sustainable Development Goals, the journal bridges knowledge gaps between fundamental research, implementation, and policy-making. Covering diverse topics such as climate change, food sustainability, environmental science, renewable energy, water, urban development, and socio-economic challenges, it contributes to the understanding and promotion of sustainable systems.
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