A review of catalyst material for hydrogen mitigation systems in nuclear facilities

IF 1.9 3区 工程技术 Q1 NUCLEAR SCIENCE & TECHNOLOGY Nuclear Engineering and Design Pub Date : 2024-07-31 DOI:10.1016/j.nucengdes.2024.113481
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Abstract

The Fukushima incident starkly underscores the imperative need to address the substantial safety risks posed by hydrogen explosions in various industrial systems utilizing hydrogen. An explosion risk arises when the concentration of hydrogen in a mixed gas surpasses 4%. Catalytic hydrogen combustion, characterized by its enhanced efficiency and safety, has emerged as a potent strategy to alleviate the detrimental effects of hydrogen explosions. This paper offers an exhaustive review of catalyst material for catalytic hydrogen combustion, encompassing diverse catalysts, and delineates the current research trajectory concerning catalyst design, fabrication, and development methodologies in a systematic manner. This review encapsulates the deleterious impacts of toxic substances—such as water vapor, carbon monoxide, iodine compounds, and fire combustion products—that may be present in nuclear facilities on catalysts and the implications of isotopic effects that warrant particular scrutiny in these settings. Finally, potential avenues for future research are suggested to alleviate hydrogen hazards in nuclear plants through the use of CHC.

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核设施氢缓和系统催化剂材料综述
福岛事件突出表明,亟需解决各种使用氢气的工业系统中氢气爆炸所带来的巨大安全风险。当混合气体中的氢浓度超过 4% 时,就会产生爆炸风险。催化氢燃烧以其更高的效率和安全性为特点,已成为减轻氢爆炸有害影响的有效策略。本文详尽综述了催化氢燃烧的催化剂材料,包括各种催化剂,并系统地勾勒了当前有关催化剂设计、制造和开发方法的研究轨迹。本综述概述了核设施中可能存在的有毒物质(如水蒸气、一氧化碳、碘化合物和火灾燃烧产物)对催化剂的有害影响,以及在这些环境中需要特别注意的同位素效应的影响。最后,提出了未来研究的潜在途径,以通过使用 CHC 来减轻核电厂中的氢危害。
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来源期刊
Nuclear Engineering and Design
Nuclear Engineering and Design 工程技术-核科学技术
CiteScore
3.40
自引率
11.80%
发文量
377
审稿时长
5 months
期刊介绍: Nuclear Engineering and Design covers the wide range of disciplines involved in the engineering, design, safety and construction of nuclear fission reactors. The Editors welcome papers both on applied and innovative aspects and developments in nuclear science and technology. Fundamentals of Reactor Design include: • Thermal-Hydraulics and Core Physics • Safety Analysis, Risk Assessment (PSA) • Structural and Mechanical Engineering • Materials Science • Fuel Behavior and Design • Structural Plant Design • Engineering of Reactor Components • Experiments Aspects beyond fundamentals of Reactor Design covered: • Accident Mitigation Measures • Reactor Control Systems • Licensing Issues • Safeguard Engineering • Economy of Plants • Reprocessing / Waste Disposal • Applications of Nuclear Energy • Maintenance • Decommissioning Papers on new reactor ideas and developments (Generation IV reactors) such as inherently safe modular HTRs, High Performance LWRs/HWRs and LMFBs/GFR will be considered; Actinide Burners, Accelerator Driven Systems, Energy Amplifiers and other special designs of power and research reactors and their applications are also encouraged.
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