Assessment of environmental impacts from authorized discharges of tritiated water from the Fukushima site to coastal and offshore regions

IF 1.9 3区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Journal of environmental radioactivity Pub Date : 2024-07-31 DOI:10.1016/j.jenvrad.2024.107507
Jakub Kaizer , Katsumi Hirose , Pavel P. Povinec
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Abstract

In August 2023, the long-planned discharging of radioactive wastewater from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) started after the confirmation of its feasibility and safety. As this water contains elevated amounts of tritium even after being diluted, a lot of resources have been invested in the monitoring of the Fukushima coastal region where the discharge outlet is located. We compare the first 3H surface activity concentrations from these measurements (up to the end of November 2023) with the available background values to evaluate a possible impact of the long-term discharging on humans and environmental levels of the radionuclide of interest in the same or nearby area. From our results, we can conclude that the joint effect of horizontal and vertical mixing has been significant enough to reduce tritium concentrations at the monitored locations in the region close to the FDNPP port two days after the end of the respective phase of the discharging beyond the detection limit of the applied analytical methods (∼0.3 Bq L−1) which is by five orders of magnitude lower than safety limit for drinking water set by the World Health Organization (WHO). Moreover, the distant correlation analysis showed that tritium concentrations at stations located further than 1.4 km were very close to pre-discharge levels (∼0.4 Bq L−1). We also estimated that the 3H activity concentration in the offshore Fukushima region would be elevated by 0.01 Bq L−1 at maximum over a year of continuous discharging, which is in concordance with the already published modeling papers and much less than the impact of the FDNPP accident in 2011.

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评估经授权从福岛核电站向沿海和近海地区排放三酸水对环境造成的影响。
2023 年 8 月,计划已久的福岛第一核电站(FDNPP)放射性废水排放在其可行性和安全性得到确认后开始实施。由于这些废水在稀释后仍含有大量氚,因此在排放口所在的福岛沿海地区投入了大量资源进行监测。我们将这些测量结果(截至 2023 年 11 月底)中的第一批 3H 表面活性浓度与现有的背景值进行比较,以评估长期排放可能对人体以及同一地区或附近地区相关放射性核素的环境水平造成的影响。根据我们的结果,我们可以得出结论,水平和垂直混合的共同作用足以使靠近国防核电站港口地区的监测点的氚浓度在相应排放阶段结束两天后降低到应用分析方法的检测限(∼0.3 Bq L-1)以外,比世界卫生组织(WHO)规定的饮用水安全限值低五个数量级。此外,远距离相关分析表明,位于 1.4 公里以外的监测站的氚浓度非常接近排放前的水平(∼0.4 Bq L-1)。我们还估计,福岛近海地区的 3H 活动浓度在连续排放一年的情况下最大将升高 0.01 Bq L-1,这与已发表的建模论文一致,且远小于 2011 年 FDNPP 事故的影响。
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来源期刊
Journal of environmental radioactivity
Journal of environmental radioactivity 环境科学-环境科学
CiteScore
4.70
自引率
13.00%
发文量
209
审稿时长
73 days
期刊介绍: The Journal of Environmental Radioactivity provides a coherent international forum for publication of original research or review papers on any aspect of the occurrence of radioactivity in natural systems. Relevant subject areas range from applications of environmental radionuclides as mechanistic or timescale tracers of natural processes to assessments of the radioecological or radiological effects of ambient radioactivity. Papers deal with naturally occurring nuclides or with those created and released by man through nuclear weapons manufacture and testing, energy production, fuel-cycle technology, etc. Reports on radioactivity in the oceans, sediments, rivers, lakes, groundwaters, soils, atmosphere and all divisions of the biosphere are welcomed, but these should not simply be of a monitoring nature unless the data are particularly innovative.
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