CH4 and CO2 Emissions From Different Tectonic Settings Along the Western Margin of the Ordos Block in China: Output and Correlation With the Regional Tectonics

IF 2.9 2区 地球科学 Q2 GEOCHEMISTRY & GEOPHYSICS Geochemistry Geophysics Geosystems Pub Date : 2024-08-14 DOI:10.1029/2024GC011661
Y. J. Cui, Y. Li, W. Zheng, J. N. Huang, Z. J. Zeng, Z. F. Liu, X. C. Zhou, F. X. Sun, Z. Y. Zou, X. Y. Si, X. Y. Li, J. G. Du
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Abstract

The investigation of tectonic controls on CH4 and CO2 emissions was conducted by measuring the fluxes of the gases in the different tectonic units along the northwestern margin of the Ordos Block in China, a region renowned for its intricate tectonic configuration. The mean fluxes of CH4 ranged from −1.5 to 1.1 mg m−2 d−1, while CO2 fluxes spanned from 2.0 to 29.2 g m−2 d−1. Notably, the Minqin, Ordos, and Haiyuan blocks primarily exhibited absorption characteristics for CH4. In contrast, within the Hetao and Yinchuan grabens, both degassing and absorption processes coexist. A striking observation was that blocks with high internal deformation exhibited significantly higher CH4 and CO2 fluxes compared to those in the stable blocks. Additionally, regions experiencing extensional deformation demonstrated greater gas emission than those undergoing compressional deformation. The spatial distribution of CH4 and CO2 fluxes at the study points exhibited a similar trend to faults in the Yinchuan Graben. Our findings revealed that CH4 and CO2 are mainly of biogenic origin, accompanied by abiotic emissions from underground. And the gas source, migration pathway, and tectonic stress were the primary factors influencing gas emission, with tectonic stress playing a pivotal role. This stress controlled the formation of tectonic structures, changed the degassing pathway, and served as the driving force for gas migration. The results of this study offer valuable insights into the mechanisms governing CH4 and CO2 emission in faulted regions. Furthermore, our results may contribute to future assessments aimed at quantifying the contribution of geological sources to greenhouse gas emissions.

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中国鄂尔多斯地块西缘不同构造背景下的甲烷和二氧化碳排放量:产出及与区域构造的相关性
通过测量中国鄂尔多斯地块西北边缘不同构造单元的气体通量,研究了构造对甲烷和二氧化碳排放的控制。甲烷的平均通量为-1.5 至 1.1 毫克/平方米/天,二氧化碳的通量为 2.0 至 29.2 克/平方米/天。值得注意的是,民勤、鄂尔多斯和海原区块主要表现出对 CH4 的吸收特征。相反,在河套地块和银川地块,脱气和吸收过程同时存在。一个显著的现象是,与稳定地块相比,内部变形较大的地块表现出更高的甲烷和二氧化碳通量。此外,与发生压缩变形的区域相比,发生伸展变形的区域气体排放量更大。研究点的CH4和CO2通量的空间分布与银川地块的断层趋势相似。研究结果表明,CH4 和 CO2 主要来源于生物,同时伴有来自地下的非生物排放。而气体来源、迁移途径和构造应力是影响气体排放的主要因素,其中构造应力起着关键作用。这种应力控制着构造结构的形成,改变了脱气途径,并成为气体迁移的驱动力。这项研究的结果为了解断层地区甲烷和二氧化碳的排放机制提供了宝贵的见解。此外,我们的研究结果可能有助于未来旨在量化地质源对温室气体排放的贡献的评估。
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来源期刊
Geochemistry Geophysics Geosystems
Geochemistry Geophysics Geosystems 地学-地球化学与地球物理
CiteScore
5.90
自引率
11.40%
发文量
252
审稿时长
1 months
期刊介绍: Geochemistry, Geophysics, Geosystems (G3) publishes research papers on Earth and planetary processes with a focus on understanding the Earth as a system. Observational, experimental, and theoretical investigations of the solid Earth, hydrosphere, atmosphere, biosphere, and solar system at all spatial and temporal scales are welcome. Articles should be of broad interest, and interdisciplinary approaches are encouraged. Areas of interest for this peer-reviewed journal include, but are not limited to: The physics and chemistry of the Earth, including its structure, composition, physical properties, dynamics, and evolution Principles and applications of geochemical proxies to studies of Earth history The physical properties, composition, and temporal evolution of the Earth''s major reservoirs and the coupling between them The dynamics of geochemical and biogeochemical cycles at all spatial and temporal scales Physical and cosmochemical constraints on the composition, origin, and evolution of the Earth and other terrestrial planets The chemistry and physics of solar system materials that are relevant to the formation, evolution, and current state of the Earth and the planets Advances in modeling, observation, and experimentation that are of widespread interest in the geosciences.
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