Study of femtosecond laser induced periodic structure on amorphous silicon films and crystallization characteristics

IF 5.4 3区 材料科学 Q2 CHEMISTRY, PHYSICAL ACS Applied Energy Materials Pub Date : 2024-09-10 DOI:10.1016/j.optlastec.2024.111764
Wei Shi , Dongfeng Qi , Wenke Wang , Zhanzhu Li , Jianguo Zhang , Hongyu Zheng , Bing Yang , Tengfei Sun , Juan Wei , Songyan Chen
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Abstract

The large area and uniform laser-induced periodic surface structure has a wide range of industrial application potential. The effect of the laser beam scanning velocity and laser fluence on the large-area fabrication of Laser-Induced Periodic Surface Structures (LIPSS), on 50 nm thickness a-Si thin films, is investigated. The results show that the formation and crystallization changes of LIPSS structure are obviously related to the scanning speed and laser fluence. In addition to surface morphology, the crystallinity of polycrystalline silicon can also be controlled by laser parameters. Based on these results, we applied direct laser induced periodic surface structuring to drive the phase transition from amorphous silicon into polycrystalline silicon. And prepare the periodic fringe structure of polycrystalline silicon with good crystallization and regular structure. By changing the polarization direction of the incident laser, the periodic surface structure with specific orientation can be obtained, and the surface of the material can be endowed with significant optical properties. When the prepared polycrystalline silicon periodic structure samples with different orientations are put into dark field microscope, the different color effects of the samples can be observed.

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非晶硅薄膜上的飞秒激光诱导周期结构及结晶特性研究
大面积、均匀的激光诱导周期表面结构具有广泛的工业应用潜力。本文研究了激光束扫描速度和激光能量对在 50 nm 厚的非晶硅薄膜上大面积制作激光诱导周期表面结构(LIPSS)的影响。结果表明,LIPSS 结构的形成和结晶变化与扫描速度和激光能量有明显的关系。除了表面形貌,多晶硅的结晶度也可以通过激光参数来控制。基于这些结果,我们应用激光直接诱导周期性表面结构来驱动从非晶硅到多晶硅的相变。并制备出结晶良好、结构规整的多晶硅周期性边缘结构。通过改变入射激光的偏振方向,可获得具有特定取向的周期性表面结构,并赋予材料表面显著的光学特性。将制备的具有不同取向的多晶硅周期结构样品放入暗视野显微镜中,可以观察到样品的不同颜色效果。
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来源期刊
ACS Applied Energy Materials
ACS Applied Energy Materials Materials Science-Materials Chemistry
CiteScore
10.30
自引率
6.20%
发文量
1368
期刊介绍: ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.
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