Effect of lubricant loading in slippery liquid-infused surface for persistent anti-icing performance

IF 6.5 2区 材料科学 Q1 CHEMISTRY, APPLIED Progress in Organic Coatings Pub Date : 2024-09-11 DOI:10.1016/j.porgcoat.2024.108797
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Abstract

Due to the vast applications in biomedical materials and aerospace industry, smart slippery liquid-infused porous surfaces (SLIPSs) have attracted remarkable attention. However, there are still challenges in the fabrication of durable SLIPS. In this work, based on linear polyurea and silicone oil, a series of durable anti-icing surface were fabricated. Based on the long-lasting secretion of lubricant, the ice adhesion strength of 60-PUa was 2.7 ± 0.5 kPa and could remain below 10 kPa even after 30 icing-deicing cycles. And the icing delay time of 60-PUa could be extended up to 870 s at a temperature of −15 °C. The introduction of large numbers of reversible hydrogen bonds in the system and silicone oil made it possible to achieve high self-healing efficiency under natural conditions. The coating system not only improved the ice removal ability, but also had excellent water-sliding properties, the droplet could slide under its own weight on 60-PUa at a tilt angle of 4.7°. This work provides an easy way to fabricate multi-functional SLIPS with durability.

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滑液注入表面的润滑剂负载对持久防冰性能的影响
由于在生物医学材料和航空航天领域的广泛应用,智能滑液注入多孔表面(SLIPSs)引起了广泛关注。然而,在制造耐用的 SLIPS 方面仍然存在挑战。本研究以线性聚脲和硅油为基础,制作了一系列耐用的防冰表面。基于润滑剂的长效分泌,60-PUa 的冰附着强度为 2.7 ± 0.5 kPa,即使在 30 次结冰-除冰循环后仍能保持在 10 kPa 以下。在温度为 -15 °C 时,60-PUa 的结冰延迟时间可延长至 870 秒。由于在系统和硅油中引入了大量可逆氢键,因此可以在自然条件下实现较高的自愈效率。该涂层系统不仅提高了除冰能力,还具有优异的水滑动性能,水滴可在 60-PUa 上以 4.7° 的倾斜角在自重作用下滑动。这项工作为制造具有耐久性的多功能 SLIPS 提供了一种简便的方法。
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来源期刊
Progress in Organic Coatings
Progress in Organic Coatings 工程技术-材料科学:膜
CiteScore
11.40
自引率
15.20%
发文量
577
审稿时长
48 days
期刊介绍: The aim of this international journal is to analyse and publicise the progress and current state of knowledge in the field of organic coatings and related materials. The Editors and the Editorial Board members will solicit both review and research papers from academic and industrial scientists who are actively engaged in research and development or, in the case of review papers, have extensive experience in the subject to be reviewed. Unsolicited manuscripts will be accepted if they meet the journal''s requirements. The journal publishes papers dealing with such subjects as: • Chemical, physical and technological properties of organic coatings and related materials • Problems and methods of preparation, manufacture and application of these materials • Performance, testing and analysis.
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