MXene/MWCNTs-based capacitive pressure sensors combine high sensitivity and wide detection range for human health and motion monitoring

IF 5.4 3区 材料科学 Q2 CHEMISTRY, PHYSICAL ACS Applied Energy Materials Pub Date : 2024-09-03 DOI:10.1016/j.sna.2024.115858
Xiaoqing Cui, Jiahui Zheng, Yichen Huang, Rui Wang, Hongyan Zhang
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Abstract

Wearable pressure sensors with exceptional performance are playing a crucial role in various fields such as electronic skin, human motion monitoring, medical diagnosis, and human-computer interaction. However, achieving both high sensitivity and a wide sensing range with simple fabrication and low cost has proven to be a significant challenge for sensors. In this study, a simple capacitive pressure sensor is proposed that multi-walled carbon nanotubes (MWCNTs) are introduced into MXene (Ti3C2TX) as a ‘bridge’. Then the electrode which has excellent conductivity is obtained by filtration of MXene solution and MXene/MWCNTs solution at intervals. Additionally, green and degradable cellulose paper is used as the dielectric layer. The fabricated pressure sensor exhibits a high sensitivity of 4.7 kPa−1 for low pressure from 0 to 1 kPa, a wide detection range of 0–700 kPa, ultra-fast response and recovery times of 46 ms and 62 ms, respectively, and an extremely low detection limit of 0.32 Pa. The sensor remains stable even after 4500 cycles and can accurately monitor the movement of the human joints. Furthermore, it can track human physiological signals, which is beneficial for medical diagnosis and disease prevention, and has significant potential for application in the wearable technology field.

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基于 MXene/MWCNT 的电容式压力传感器兼具高灵敏度和宽检测范围,可用于人体健康和运动监测
性能卓越的可穿戴压力传感器在电子皮肤、人体运动监测、医疗诊断和人机交互等多个领域发挥着至关重要的作用。然而,如何在实现高灵敏度和宽传感范围的同时,做到制作简单、成本低廉,已被证明是传感器面临的一项重大挑战。本研究提出了一种简单的电容式压力传感器,即在 MXene(Ti3C2TX)中引入多壁碳纳米管(MWCNT)作为 "桥"。然后将 MXene 溶液和 MXene/MWCNTs 溶液间隔过滤,就得到了导电性极佳的电极。此外,还使用了可降解的绿色纤维素纸作为电介质层。制成的压力传感器在 0 至 1 kPa 的低压下具有 4.7 kPa-1 的高灵敏度、0 至 700 kPa 的宽检测范围、分别为 46 毫秒和 62 毫秒的超快响应和恢复时间以及 0.32 Pa 的极低检测限。该传感器即使在循环使用 4500 次后仍能保持稳定,并能准确监测人体关节的运动。此外,它还能跟踪人体生理信号,有利于医疗诊断和疾病预防,在可穿戴技术领域具有巨大的应用潜力。
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来源期刊
ACS Applied Energy Materials
ACS Applied Energy Materials Materials Science-Materials Chemistry
CiteScore
10.30
自引率
6.20%
发文量
1368
期刊介绍: ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.
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