Investigation of bubble formation dynamics of gas-non-Newtonian liquid two-phase flow in a flow-focusing generator

Abstract

In the present study, we explore the dynamics of bubble formation in a flow-focusing device designed for gas-non-Newtonian liquid two-phase flow. The flow-focusing device with a cross-section of a square (300 μm × 300 μm) is constructed on polydimethylsiloxane using lithographic techniques and subsequently sealed with polymethylmethacrylate. A high-speed camera is employed to document the process of bubble formation during the experiment, complemented by computational fluid dynamics methods for an in-depth analysis. The gas is nitrogen, and the liquid is sodium carboxymethyl cellulose solutions with mass fractions of 0.1, 0.2, and 0.3%, respectively. The inlet flow rates of gas and liquid are set at 1–2 ml/min in the simulation and the experiment, and the observed flow patterns are all slug flows. Experimental findings suggest that the duration of bubble formation can be bifurcated into two distinct parts. The first part is predominantly influenced by the velocity of the inlet gas, and the correlation coefficient between velocity and time is −0.56, while the second part is impacted by the shear-thinning properties of the liquid, which are correlated with the flow index and viscosity coefficient of the non-Newtonian liquids, and the correlation coefficients are −0.47 and 0.48, respectively. The computational fluid dynamics results of gas-non-Newtonian liquid two-phase flow with gas and liquid flow rates of 2 ml/min corroborate that the manifestation of the aforementioned time segmentation phenomenon primarily depends on the vortex intensity at the bubble’s head and the orientation of pressure gradients. When the bubble neck size approaches 0, the viscosity of the surrounding liquid decreases rapidly, and alterations in the velocity field near the bubble neck trigger fluctuations in the viscosity of the non-Newtonian liquid, thereby influencing the bubble formation process.