Zeolite-based materials for greenhouse gas capture and conversion

IF 10.4 1区化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Science China Chemistry Pub Date : 2024-09-09 DOI:10.1007/s11426-024-2287-6

Qiang Zhang, Jialiang Li, Li Li, Jihong Yu

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Abstract

The global warming caused by greenhouse gas emissions, principally carbon dioxide (CO₂) and methane (CH₄), has become a great threat to human survival. The capture and conversion of CO₂ and CH₄ not only provide an effective method to reduce the greenhouse gas emissions towards achieving carbon neutrality but also produce sustainable chemicals and fuels to meet the increasing demand for chemicals and energy. Zeolite-based materials are excellent adsorbents and catalysts for CO₂ and CH₄ capture and conversion. In this mini-review, we present the recent progress in zeolite-based materials for CO₂ and CH₄ capture and conversion. We first discuss the key factors of zeolites on the CO₂ and CH₄ adsorption performance. Then, we demonstrate the catalytic conversion of CO₂ and CH₄ into value-added chemicals, including hydrocarbons, oxygenates, and syngas. Finally, we provide an outlook regarding the opportunities and challenges for the capture and conversion of CO₂ and CH₄ towards achieving carbon neutrality and sustainable development.

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用于温室气体捕获和转化的沸石基材料

温室气体排放（主要是二氧化碳（CO2）和甲烷（CH4））造成的全球变暖已成为人类生存的巨大威胁。二氧化碳和甲烷的捕获和转化不仅是减少温室气体排放、实现碳中和的有效方法，还能生产可持续的化学品和燃料，以满足日益增长的化学品和能源需求。沸石基材料是二氧化碳和甲烷捕集与转化的优良吸附剂和催化剂。在这篇微型综述中，我们将介绍用于二氧化碳和甲烷捕集与转化的沸石基材料的最新进展。我们首先讨论了沸石对二氧化碳和甲烷吸附性能影响的关键因素。然后，我们演示了将 CO2 和 CH4 催化转化为高附加值化学品（包括碳氢化合物、含氧化合物和合成气）的过程。最后，我们展望了二氧化碳和甲烷捕集与转化在实现碳中和与可持续发展方面的机遇与挑战。

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来源期刊

Science China Chemistry CHEMISTRY, MULTIDISCIPLINARY-

CiteScore

14.40

自引率

7.30%

发文量

3787

审稿时长

2.2 months

期刊介绍： Science China Chemistry, co-sponsored by the Chinese Academy of Sciences and the National Natural Science Foundation of China and published by Science China Press, publishes high-quality original research in both basic and applied chemistry. Indexed by Science Citation Index, it is a premier academic journal in the field. Categories of articles include: Highlights. Brief summaries and scholarly comments on recent research achievements in any field of chemistry. Perspectives. Concise reports on thelatest chemistry trends of interest to scientists worldwide, including discussions of research breakthroughs and interpretations of important science and funding policies. Reviews. In-depth summaries of representative results and achievements of the past 5–10 years in selected topics based on or closely related to the research expertise of the authors, providing a thorough assessment of the significance, current status, and future research directions of the field.