Weak decays in superheavy nuclei

A. Ravlić, W. Nazarewicz
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Abstract

Superheavy nuclei represent the heaviest atoms and nuclides known at the limit of mass and charge. The observed superheavy nuclei are all proton-rich; they decay primarily by emitting $\alpha$ particles and fission, with a possible small electron capture (EC) branch. Due to the huge atomic numbers and associated relativistic effects, EC-decays of superheavy systems are expected to differ from what is known in lighter nuclei. In this paper, using the quantified relativistic nuclear density functional theory and the quasiparticle random-phase approximation with the interaction optimized to experimental $\beta^-$-decay half-lives and Gamow-Teller resonance energies, we study the EC/$\beta^\pm$-decays in $Z = 101-118$ nuclei. Both allowed ($1^+$) and first-forbidden ($0^-, 1^-$ and $2^-$) transitions are considered. We show that the first-forbidden $1^-$ transitions dominate the decay rates in almost all studied nuclei. For proton-rich nuclei, EC dominates over $\beta^+$ decay. We identify 44 nuclei with EC/$\beta^+$ branching ratio larger than 5\%, indicating a possible competition with $\alpha$-decay and spontaneous fission channels.
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超重核中的弱衰变
超重核代表了已知质量和电荷极限的最重原子和核素。观测到的超重原子核都富含质子;它们主要通过发射α粒子和裂变衰变,也可能有小的电子俘获(EC)分支。由于巨大的原子序数和相关的相对论效应,超重原子核系统的电子俘获衰变预计将不同于已知的轻原子核。在本文中,我们使用量化的相对论核密度泛函理论和准方随机相近似,并根据实验$\beta^-$-衰变半衰期和伽莫-泰勒共振能量对相互作用进行了优化,研究了$Z = 101-118$原子核中的EC/$\beta^\pm$-衰变。我们考虑了允许的(1^+$)和第一禁止的(0^-、1^-$ 和 2^-$)转变。我们的研究表明,在几乎所有被研究的原子核中,首先被禁止的 1^-$ 转换都主导着衰变速率。对于富质子原子核,EC衰变比$\beta^+$衰变占主导地位。我们发现有44个原子核的EC/$\beta^+$分支比大于5%,这表明可能存在与$\alpha$衰变和自发裂变通道的竞争。
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