High-precision mass measurements of the ground and isomeric states in $^{124,125}$Ag

J. Ruotsalainen, D. A. Nesterenko, M. Stryjczyk, A. Kankainen, L. Al Ayoubi, O. Beliuskina, L. Canete, P. Chauveau, R. P. de Groote, P. Delahaye, T. Eronen, M. Flayol, Z. Ge, S. Geldhof, W. Gins, M. Hukkanen, A. Jaries, D. Kahl, D. Kumar, I. D. Moore, S. Nikas, H. Penttilä, D. Pitman-Weymouth, A. Raggio, S. Rinta-Antila, A. de Roubin, M. Vilen, V. Virtanen, M. Winter
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Abstract

The masses of the ground and isomeric states in $^{124,125}$Ag have been measured using the phase-imaging ion-cyclotron-resonance technique at the JYFLTRAP double Penning trap mass spectrometer. The ground states of $^{124}$Ag and $^{125}$Ag were found to be 30(250) keV and 250(430) keV less bound but 36 and 110 times more precise than in the Atomic Mass Evaluation 2020, respectively. The excitation energy of $^{124}$Ag$^{m}$, ${E_x = 188.2(25)}$ keV, was determined for the first time. The new precise mass values have been utilised to study the evolution of nuclear structure via two-neutron separation energies. The impact on the astrophysical rapid neutron capture process has been investigated via neutron-capture reaction rate calculations. The precision measurements indicate a more linear trend in two-neutron separation energies and reduce the mass-related uncertainties for the neutron-capture rate of $^{124}$Ag$(n,\gamma)^{125}$Ag by a factor of around 100. The new mass values also improve the mass of $^{123}$Pd, previously measured using $^{124}$Ag as a reference.
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对 $^{124,125}$Ag 的基态和异构态进行高精度质量测量
在 JYFLTRAP 双潘宁陷阱质谱仪上,利用相位成像离子-回旋共振技术测量了 $^{124,125}$Ag 的基态和异构态的质量。结果发现,$^{124}$Ag 和 $^{125}$Ag 的基态束缚分别比原子质量评估 2020 中的结果低 30(250) keV 和 250(430) keV,但精确度分别高出 36 倍和 110 倍。首次测定了 $^{124}$Ag$^{m}$ 的激发能量 ${E_x = 188.2(25)}$keV 。新的精确质量值被用来研究核结构通过双中子分离能量的演变。通过中子俘获反应速率计算,研究了对天体物理快速中子俘获过程的影响。精确测量结果表明,双中子分离能的趋势更加线性,并将$^{124}$Ag$(n,\gamma)^{125}$Ag的中子俘获率的质量相关不确定性降低了约100倍。新的质量值还改进了$^{123}$Pd的质量,以前的测量是以$^{124}$Ag作为参考的。
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