Gate induced metallicity and absence of superconductivity in BSTO/LCO heterostructure

IF 2.8 3区 物理与天体物理 Q2 PHYSICS, CONDENSED MATTER Physica B-condensed Matter Pub Date : 2024-09-12 DOI:10.1016/j.physb.2024.416527
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Abstract

We fabricated Ba0.8Sr0.2TiO3 (BSTO)/La2CuO4 (LCO) heterostructure on SrTiO3 (STO) substrate and investigated its structure and physical properties. X-ray diffraction and reciprocal space mapping confirm the epitaxial growth of BSTO/LCO/STO heterostructure. X-ray photoelectron spectroscopy and UV–Visible spectroscopy measurements reveal a straddling band alignment of the BSTO/LCO heterojunction. Such band alignment facilitates the accumulation of both electrons and holes at the interface. Their movement depends on the direction of the internal field of the BSTO film. Electrical transport measurements have revealed a signature of insulator-to-metal transition (IMT) in response to applied gate voltages ±Vg. Hall measurements confirm the presence of electron and hole type charge carriers under +Vg and −Vg, respectively. We have proposed a screening mechanism linked to the polarization state of the BSTO film to explain the observed IMT.

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BSTO/LCO 异质结构中的栅极诱导金属性和无超导现象
我们在SrTiO3(STO)衬底上制备了Ba0.8Sr0.2TiO3(BSTO)/La2CuO4(LCO)异质结构,并对其结构和物理性质进行了研究。X 射线衍射和倒易空间图证实了 BSTO/LCO/STO 异质结构的外延生长。X 射线光电子能谱和紫外-可见光谱测量揭示了 BSTO/LCO 异质结的跨带排列。这种带排列有利于电子和空穴在界面上聚集。它们的移动取决于 BSTO 薄膜内部场的方向。电输运测量显示,在施加栅极电压 ±Vg 时,会出现绝缘体到金属的转变(IMT)。霍尔测量证实,在 +Vg 和 -Vg 下分别存在电子和空穴型电荷载流子。我们提出了一种与 BSTO 薄膜极化状态相关的屏蔽机制,以解释观察到的 IMT。
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来源期刊
Physica B-condensed Matter
Physica B-condensed Matter 物理-物理:凝聚态物理
CiteScore
4.90
自引率
7.10%
发文量
703
审稿时长
44 days
期刊介绍: Physica B: Condensed Matter comprises all condensed matter and material physics that involve theoretical, computational and experimental work. Papers should contain further developments and a proper discussion on the physics of experimental or theoretical results in one of the following areas: -Magnetism -Materials physics -Nanostructures and nanomaterials -Optics and optical materials -Quantum materials -Semiconductors -Strongly correlated systems -Superconductivity -Surfaces and interfaces
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