Observation of near-scission “polar” and “equatorial” proton emission in heavy-ion induced fission

IF 5.4 3区 材料科学 Q2 CHEMISTRY, PHYSICAL ACS Applied Energy Materials Pub Date : 2024-09-11 DOI:10.1016/j.physletb.2024.139014
Pawan Singh , Y.K. Gupta , G.K. Prajapati , B.N. Joshi , V.G. Prajapati , N. Sirswal , K. Ramachandran , A.S. Pradeep , V.S. Dagre , M. Kumar , A. Jhingan , N. Deshmukh , B.V. John , B.K. Nayak , D.C. Biswas , R.K. Choudhury
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Abstract

Proton and α-particle energy spectra were measured in coincidence with fission fragments at different relative angles in 16O (96 MeV) + 232Th reaction. The multiplicity spectra were analyzed within the framework of a Moving Source Disentangling Analysis (MSDA) to determine contributions from different emission stages. The MSDA conclusively shows “Near Scission Emission (NSE)” as an essential component in the multiplicity spectra. In contrast to NSE α particles which emit mainly perpendicular (“equatorial emission”), the NSE protons are observed to be emitted perpendicular as well as parallel (“polar emission”) to the fission axis with similar intensities (~20% for each). Thus, around 40% of total pre-scission protons are emitted near the scission stage, whereas the same fraction for α particles is only around 10%. The inevitable presence of “polar” and “equatorial” NSE protons in a heavy-ion induced fission has been observed for the first time. Present results open up a new avenue to study the heavy-ion induced fission dynamics.

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观测重离子诱导裂变中质子的近裂变 "极 "和 "赤道 "发射
在 16O (96 MeV) + 232Th 反应中,质子和 α 粒子能谱与裂变碎片以不同的相对角度同时进行了测量。在移动源分解分析(MSDA)的框架内对多重性光谱进行了分析,以确定不同发射阶段的贡献。MSDA 明确显示 "近裂变发射(NSE)"是倍率光谱中的重要组成部分。与主要垂直发射("赤道发射")的 NSE α 粒子不同,NSE 质子的发射既垂直于裂变轴,也平行于裂变轴("极性发射"),且强度相似(各占约 20%)。因此,在裂变阶段附近发射的质子约占裂变前质子总数的 40%,而 α 粒子的这一比例仅为 10%左右。在重离子诱导的裂变中不可避免地存在 "极性 "和 "赤道 "NSE质子,这还是第一次被观测到。目前的结果为研究重离子诱导裂变动力学开辟了一条新途径。
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来源期刊
ACS Applied Energy Materials
ACS Applied Energy Materials Materials Science-Materials Chemistry
CiteScore
10.30
自引率
6.20%
发文量
1368
期刊介绍: ACS Applied Energy Materials is an interdisciplinary journal publishing original research covering all aspects of materials, engineering, chemistry, physics and biology relevant to energy conversion and storage. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials, engineering, physics, bioscience, and chemistry into important energy applications.
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