Effect of hybrid lead-PVA fibers on microstructure and radiation shielding properties of high-performance concrete

Abstract

With the widespread application of nuclear technology in the medical and energy fields, the demand for efficient radiation shielding materials is increasing. Employing only lead or polyvinyl alcohol (PVA) fiber reinforcement cannot achieve improvements in the brittleness of high-performance concrete (HPC) while also enhancing radiation shielding efficiency and mechanical properties. This study develops a novel HPC for radiation attenuation, incorporating magnetite as the aggregate and reinforced with hybrid lead-PVA fibers (RSHPC). The synergistic effects of various proportions of hybrid lead-PVA fibers on the mechanical properties, three-dimensional microstructure, pore structure, and interfacial transition zone (ITZ) were investigated. In addition, the radiation attenuation capacities of RSHPC with different hybrid lead-PVA fiber proportions were evaluated through experimental and simulation analysis. The results show that hybrid lead-PVA fibers notably improve the air-void structure of RSHPC. The incorporation of PVA fibers, by improving the ITZ of matrix, effectively mitigates the negative impact of lead fibers on mechanical performance. The refinement of pore structure and the introduction of light and heavy nuclides lead to a significant enhancement in the gamma-ray and neutron radiation attenuation capabilities of RSHPC. Utilizing X-ray computed tomography (X-CT) for three-dimensional reconstruction further indicates the optimization impact of hybrid lead-PVA fibers on the microstructure, notably in the improvement of pore distribution and fiber dispersion, thus enhancing the overall properties and radiation attenuation performance of RSHPC.