Measurement of fast neutron induced (n,γ) reaction cross-section of 68Zn, 96Zr, 121Sb and 123Sb in the energy range of 1 to 2 MeV

Abstract

The (n,γ) reaction cross-section for the elements ⁶⁸Zn, ⁹⁶Zr, ¹²¹Sb and ¹²³Sb, present in the reactor structural/shielding materials, was measured by neutron activation technique in the neutron energy region of 1–2 MeV as very limited data is available in this energy range. Further, the neutron spectrum peaks in this energy region for the fast breeder reactors and proposed accelerator driven sub-critical systems. The natural strontium (^natSr) element was used as a neutron flux monitor by considering effective combined reaction cross-section for ⁸⁶Sr(n,γ)⁸⁷Sr^m and ⁸⁷Sr(n,n′)⁸⁷Sr^m reactions. The pellets of mixture of sample and monitor were irradiated by a quasi-mono energetic fast neutron beam, generated by ⁷Li(p,n)⁷Be reaction at FOTIA, Bhabha Atomic Research Centre, Mumbai, India. The activity of activation products was measured by off-line gamma-ray spectrometry using High Purity Germanium Detector (HPGe). The present data with improved uncertainty and covariance analysis enhance the cross-section data base for better constraining the evaluated data and theoretical models. The theoretical (n,γ) reaction cross-sections were calculated using TALYS 1.96, which could reasonably explain the present data with the Fermi gas level density prescription.