Analysis of the National Air Pollutant Emissions Inventory (CAPSS 2018) Data and Assessment of Emissions Based on Air Quality Modeling in the Republic of Korea

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2022-12-01 DOI:10.5572/ajae.2022.084
Seong-woo Choi, Hyeonjeong Cho, Yumi Hong, Hee-ji Jo, Min Park, Hyeon-ji Lee, Ye-ji Choi, Ho-hyun Shin, Dongjae Lee, Eunji Shin, Wooseung Baek, Sung-kyu Park, Eunhye Kim, Hyung-cheon Kim, Seung-joo Song, Yunseo Park, Jinsik Kim, Jihye Baek, Jinsik Kim, Chul Yoo
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Abstract

According to the 2018 National Air Pollutant Emissions Inventory (NEI), air pollutant emissions in the Republic of Korea comprised 808,801 tons of CO, 1,153,265 tons of NOX, 300,979 tons of SOX, 617,481 tons of TSP, 232,993 tons of PM10, 98,388 tons of PM2.5, 15,562 tons of black carbon (BC), 1,035,636 tons of VOCs, and 315,975 tons of NH3. As for national emission contributions to primary PM2.5 and PM precursors (NOX, SOX, VOCs, and NH3), major source categories were the road sector for NOX, the industry sector for SOX and PM2.5, and the everyday activities and others sector for VOCs and NH3. In the case of emissions by region, the largest amount of NOX was emitted from the Seoul Metropolitan Areas (SMA; Seoul, Incheon, and Gyeonggi-do, hereafter SMA) and the largest amounts of SOX, PM2.5, VOCs, and NH3 were from the Yeongnam region. A 3D chemical transport modeling system was used to examine the uncertainty of the national air pollutant emissions based on the National Emission and Air Quality Assessment System (NEAS). Air quality was simulated using CAPSS 2018, and the simulation data were compared with observed concentrations to examine the uncertainties of the current emissions. These data show that emissions from five si (cities) (Pohang, Yeosu, Gwangyang, Dangjin, and Ulsan) need to be improved. Most of all, it is necessary to examine the emissions from places of business that use anthracite, which is the major PM2.5 emission source, as fuel in these areas.

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大韩民国国家空气污染物排放清单(CAPSS 2018)数据分析及基于空气质量模型的排放评估
根据《2018 年全国大气污染物排放清单》(NEI),大韩民国的大气污染物排放量包括 808,801 吨 CO、1,153,265 吨 NOX、300,979 吨 SOX、617,481 吨 TSP、232,993 吨 PM10、98,388 吨 PM2.5、15,562 吨黑碳(BC)、1,035,636 吨 VOC 和 315,975 吨 NH3。至于国家对初级 PM2.5 和 PM 前体(氮氧化物、硫氧化物、挥发性有机化合物和 NH3)的排放贡献,主要来源类别是道路部门的氮氧化物、工业部门的硫氧化物和 PM2.5,以及日常活动和其他部门的挥发性有机化合物和 NH3。就各地区的排放量而言,最大的 NOX 排放量来自首尔首都圈(SMA;首尔、仁川和京畿道,以下简称 SMA),最大的 SOX、PM2.5、VOCs 和 NH3 排放量来自岭南地区。在国家排放和空气质量评估系统(NEAS)的基础上,使用三维化学传输模型系统对全国空气污染物排放的不确定性进行了研究。使用 CAPSS 2018 对空气质量进行了模拟,并将模拟数据与观测浓度进行了比较,以检验当前排放量的不确定性。这些数据表明,五个城市(浦项、丽水、光阳、唐津和蔚山)的排放量需要改善。最重要的是,有必要检查这些地区使用无烟煤(PM2.5 的主要排放源)作为燃料的营业场所的排放情况。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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