Semi-supervised comparative learning compensation method for chemical gas sensor drift.

IF 3.8 2区 化学 Q1 BIOCHEMICAL RESEARCH METHODS Analytical and Bioanalytical Chemistry Pub Date : 2024-12-01 Epub Date: 2024-10-21 DOI:10.1007/s00216-024-05577-2
Lijian Xiong, Meng Wang, Zhaoshuai Zhu, Meng He, Yuxin Hou, Xiuying Tang
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Abstract

The gradual and unpredictable variation in chemo-sensory signal responses when exposed to the same analyte under identical conditions, commonly referred to as sensor drift, has long been recognized as one of the most serious challenges faced by chemical sensors. The traditional drift compensation method is both labor-intensive and expensive, as it requires frequent collection and labeling of gas samples for recalibration. Introducing a small number of meaningful drift calibration samples can be an attractive strategy to reduce the computational load and improve the performance of the updated classifier. However, under the influence of drift, new challenges arise due to the difference in the distribution of source and target domain data. This paper proposes a novel algorithm framework called semi-supervised contrastive learning drift compensation (SSCLDC). The framework automatically extracts high-level abstract features based on a multilayer perceptron to better represent the structure of the source data. In addition, to address the issue of data distribution differences caused by drift between the source and target domains. We add a small number of reference sample pairs into the training for semi-supervised learning. Combining a contrastive loss function that can represent the matching degree of paired samples effectively overcomes the problem of sensor drift. The Kennard-Stone sequential algorithm is used to select the representative reference sample from the set of candidate reference samples. Experiments conducted on a widely used long-term chemical gas sensor drift dataset demonstrate that the proposed method outperforms several classic drift compensation techniques, highlighting its effectiveness and practical applicability.

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化学气体传感器漂移的半监督比较学习补偿方法。
化学传感器在相同的条件下接触相同的分析物时,其化学传感信号反应会逐渐发生不可预测的变化,这种变化通常被称为传感器漂移,这早已被公认为是化学传感器所面临的最严峻挑战之一。传统的漂移补偿方法既耗费人力,又成本高昂,因为它需要频繁地采集和标记气体样本进行重新校准。引入少量有意义的漂移校准样本是一种有吸引力的策略,可以减少计算负荷并提高更新分类器的性能。然而,在漂移的影响下,由于源域和目标域数据分布的不同,会产生新的挑战。本文提出了一种名为半监督对比学习漂移补偿(SSCLDC)的新型算法框架。该框架基于多层感知器自动提取高级抽象特征,以更好地表示源数据的结构。此外,为了解决源域和目标域之间漂移造成的数据分布差异问题。我们在半监督学习的训练中加入了少量参考样本对。结合能表示配对样本匹配度的对比损失函数,可以有效克服传感器漂移问题。Kennard-Stone 序列算法用于从候选参考样本集中选择具有代表性的参考样本。在一个广泛使用的长期化学气体传感器漂移数据集上进行的实验表明,所提出的方法优于几种经典的漂移补偿技术,突出了其有效性和实用性。
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来源期刊
CiteScore
8.00
自引率
4.70%
发文量
638
审稿时长
2.1 months
期刊介绍: Analytical and Bioanalytical Chemistry’s mission is the rapid publication of excellent and high-impact research articles on fundamental and applied topics of analytical and bioanalytical measurement science. Its scope is broad, and ranges from novel measurement platforms and their characterization to multidisciplinary approaches that effectively address important scientific problems. The Editors encourage submissions presenting innovative analytical research in concept, instrumentation, methods, and/or applications, including: mass spectrometry, spectroscopy, and electroanalysis; advanced separations; analytical strategies in “-omics” and imaging, bioanalysis, and sampling; miniaturized devices, medical diagnostics, sensors; analytical characterization of nano- and biomaterials; chemometrics and advanced data analysis.
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