Topological phase transitions via attosecond x-ray absorption spectroscopy.

Juan F P Mosquera, Giovanni Cistaro, Mikhail Malakhov, Emilio Pisanty, Alexandre Dauphin, Luis Plaja, Alexis Chacón, Maciej Lewenstein, Antonio Picón
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Abstract

We present a numerical experiment that demonstrates the possibility to capture topological phase transitions via an x-ray absorption spectroscopy scheme. We consider a Chern insulator whose topological phase is tuned via a second-order hopping. We perform time-dynamics simulations of the out-of-equilibrium laser-driven electron motion that enables us to model a realistic attosecond spectroscopy scheme. In particular, we use an ultrafast scheme with a circularly polarized IR pump pulse and an attosecond x-ray probe pulse. A laser-induced dichroism-type spectrum shows a clear signature of the topological phase transition. We are able to connect these signatures with the Berry structure of the system. This work extend the applications of attosecond absorption spectroscopy to systems presenting a non-trivial topological phase.

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通过阿秒 X 射线吸收光谱实现拓扑相变。
我们提出了一个数值实验,证明了通过 X 射线吸收光谱方案捕捉拓扑相变的可能性。我们考虑了一个通过二阶跳变调整拓扑相位的切尔绝缘体。我们对失衡激光驱动的电子运动进行了时间动力学模拟,从而建立了一个现实的阿秒光谱方案模型。特别是,我们使用了一种具有圆偏振红外泵浦脉冲和阿秒 x 射线探针脉冲的超快方案。激光诱导的二色性光谱显示了拓扑相变的明显特征。我们能够将这些特征与系统的贝里结构联系起来。这项工作将阿秒吸收光谱的应用扩展到了呈现非三维拓扑相位的系统。
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