Stochastic migrations of Marangoni surfers between two lobes of a dumbbell-shaped confinement†

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Soft Matter Pub Date : 2024-10-22 DOI:10.1039/D4SM00914B
Alakesh Upadhyaya and V. S. Akella
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Abstract

We report an experimental investigation on the stochastic migration dynamics of Marangoni surfers (camphor-infused paper disks) between the two lobes of a dumbbell-shaped chamber. We characterize the migration dynamics using survival analysis of a configuration, wherein a configuration represents a distinct distribution of disks between the lobes. We observe that a configuration's stability decreases with increasing pairwise interactions. Consequently, the configuration with equal partitioning of disks between the lobes—that is exactly one-half of disks in each lobe for even-numbered systems but with one extra disk in either of the lobes for odd-numbered systems—has the lowest pairwise interactions, thus is always the most stable configuration. Furthermore, all configurations exhibit a stretched exponential decay with time, which is ascribed to a disk's activity decay with time or “aging”—a phenomenon validated by modeling a camphor disk as a chiral active particle (CAP) as initially proposed by Cruz et al.

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马兰戈尼冲浪者在哑铃形封闭体两个叶片之间的随机迁移。
我们报告了一项关于马兰戈尼冲浪者(注入樟脑的纸盘)在哑铃形腔室两叶之间随机迁移动力学的实验研究。我们通过对构型的生存分析来描述迁移动力学,其中构型代表了纸盘在两叶之间的独特分布。我们观察到,一个构型的稳定性会随着成对相互作用的增加而降低。因此,各叶之间磁盘分配相等的配置--即偶数系统每个叶中的磁盘数正好为二分之一,而奇数系统任一叶中多出一个磁盘--具有最低的成对相互作用,因此总是最稳定的配置。此外,所有构型都会随时间呈现拉伸指数衰减,这是由于磁盘的活性会随时间衰减或 "老化"--克鲁兹(Cruz)等人最初提出的手性活性粒子(CAP)模型验证了这一现象。
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来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Where physics meets chemistry meets biology for fundamental soft matter research.
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