Stochastic migrations of Marangoni surfers between two lobes of a dumbbell-shaped confinement†

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Soft Matter Pub Date : 2024-10-22 DOI:10.1039/D4SM00914B
Alakesh Upadhyaya and V. S. Akella
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Abstract

We report an experimental investigation on the stochastic migration dynamics of Marangoni surfers (camphor-infused paper disks) between the two lobes of a dumbbell-shaped chamber. We characterize the migration dynamics using survival analysis of a configuration, wherein a configuration represents a distinct distribution of disks between the lobes. We observe that a configuration's stability decreases with increasing pairwise interactions. Consequently, the configuration with equal partitioning of disks between the lobes—that is exactly one-half of disks in each lobe for even-numbered systems but with one extra disk in either of the lobes for odd-numbered systems—has the lowest pairwise interactions, thus is always the most stable configuration. Furthermore, all configurations exhibit a stretched exponential decay with time, which is ascribed to a disk's activity decay with time or “aging”—a phenomenon validated by modeling a camphor disk as a chiral active particle (CAP) as initially proposed by Cruz et al.

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马兰戈尼冲浪者在哑铃形封闭体两个叶片之间的随机迁移。
我们报告了一项关于马兰戈尼冲浪者(注入樟脑的纸盘)在哑铃形腔室两叶之间随机迁移动力学的实验研究。我们通过对构型的生存分析来描述迁移动力学,其中构型代表了纸盘在两叶之间的独特分布。我们观察到,一个构型的稳定性会随着成对相互作用的增加而降低。因此,各叶之间磁盘分配相等的配置--即偶数系统每个叶中的磁盘数正好为二分之一,而奇数系统任一叶中多出一个磁盘--具有最低的成对相互作用,因此总是最稳定的配置。此外,所有构型都会随时间呈现拉伸指数衰减,这是由于磁盘的活性会随时间衰减或 "老化"--克鲁兹(Cruz)等人最初提出的手性活性粒子(CAP)模型验证了这一现象。
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来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Soft Matter is an international journal published by the Royal Society of Chemistry using Engineering-Materials Science: A Synthesis as its research focus. It publishes original research articles, review articles, and synthesis articles related to this field, reporting the latest discoveries in the relevant theoretical, practical, and applied disciplines in a timely manner, and aims to promote the rapid exchange of scientific information in this subject area. The journal is an open access journal. The journal is an open access journal and has not been placed on the alert list in the last three years.
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