Exploring ultrafine particle emission characteristics from in-use light-duty diesel trucks in China using a portable measurement system.

Abstract

Diesel vehicle exhaust is one of the major contributors to ultrafine particles (UFPs) in urban areas in China. However, there is still a lack of knowledge about UFPs emission characteristics from current in-use diesel vehicles. This study has carried out an on-road test of 10 in-use Light-duty Diesel Trucks (LDDTs) with different emission control standards in China using a self-established portable measurement system based on the Electronic Low-pressure Impactor (ELPI) and characterized the ultrafine particle number (PN) concentration, particle size distribution and metal element contents. The results revealed a significant reduction of 93.37% in the average PN_0.1 emission factor of LDDTs from China IV to China VI. Notably, LDDTs compliant with the China VI vehicle emission control standard exhibited the lowest PN_0.1 and PM_0.1 emission factors, measuring 4.991×10¹⁴ #/km and 0.627 g/km, respectively. By taking into account emissions under real driving conditions, we found that the PN emission rates grow with the increase of the Vehicle Specific Power (VSP). The cold-start phase had higher PN emissions than the hot-start phase, with 8590, 1890, 477, and 22 times higher than those of the ambient air (1.18×10⁵ #/cm³), respectively. The installation of Diesel Particulate Filter (DPF) can decrease UFPs by more than 99.8%, while the PN emission factor during the DPF regeneration stage (1.85×10¹⁶ #/km) increased by 5 orders of magnitude that of the DPF normal works (7.51×10¹¹ #/km). Metal element contents analysis shows that Fe, Ca, Al and Mg are the dominant elements in UFPs of LDDT exhaust gas, but the element of Ni is slightly increasing in a China VI, possibly due to the new automotive engine exhaust manifolds being made of Ni instead of cast iron for the purpose of having more high-temperature resistance. Our study demonstrates the importance of monitoring and routine maintenance of exhaust after-treatment systems.