Legacy of aerosol radiative effect predominates daytime dust loading evolution

Abstract

Dust radiative effect imposes pronounced perturbations on planetary boundary layer (PBL) development. In turn, the modified PBL characteristics and circulation fields regulate subsequent dust processes, which have not been explored sufficiently. In this study, parallel experiments are designed to isolate the instant, legacy and nonlinear impacts of aerosol radiative effect on daytime dust storm evolution over the Tarim Basin. During a typical dust storm event, legacy radiative effect is found to dominate dust loading dynamics and modulates mean dust burden by more than 16 % in the central basin and − 41 % in the marginal basin. Specifically, the dust column concentration increases in central regions but decreases in marginal regions. Dust aerosols cause opposite heating rate distributions and PBL structure between the central and marginal regions through altering radiative balance. Dust-induced cooling effect in the marginal regions leads to PBL suppression and attenuates entrainment mixing. Negative net heating also results in lowered potential temperature, elevated air pressure and thus increases their horizontal gradients. Accordingly, wind speeds are amplified through geostrophic and thermal wind effects, which further accelerate deposition rates, and eventually weaken dust suspension. In the central basin, dust plumes stimulate a warm mixing layer and unstable entrainment zone, which inhibit dry deposition removal and favor dust accumulation in the atmosphere. Our study highlights the importance of accounting PBL dynamics and geostrophic balance in quantifying the impacts of preceding radiative effect on subsequent dust evolution.