Spectrally Tunable Ultrafast Long Wave Infrared Detection at Room Temperature.

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nano Letters Pub Date : 2024-11-06 DOI:10.1021/acs.nanolett.4c03832
Tianyi Guo, Sayan Chandra, Arindam Dasgupta, Muhammad Waqas Shabbir, Aritra Biswas, Debashis Chanda
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Abstract

Room-temperature longwave infrared (LWIR) detectors are preferred over cryogenically cooled solutions due to the cost effectiveness and ease of operation. The performance of present uncooled LWIR detectors such as microbolometers, is limited by reduced sensitivity, slow response time, and the lack of dynamic spectral tunability. Here, we present a graphene-based efficient room-temperature LWIR detector with high detectivity and fast response time utilizing its tunable optical and electronic characteristics. The inherent weak light absorption is enhanced by Dirac plasmons on the patterned graphene coupled to an optical cavity. The absorbed energy is converted into photovoltage by the Seebeck effect with an asymmetric carrier generation environment. Further, dynamic spectral tunability in the 8-12 μm LWIR band is achieved by electrostatic gating. The proposed detection platform paves the path to a fresh generation of uncooled graphene-based LWIR photodetectors for wide ranging applications such as molecular sensing, medical diagnostics, military, security and space.

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室温下光谱可调谐超快长波红外探测。
与低温冷却解决方案相比,室温长波红外(LWIR)探测器因其成本效益和操作简便而更受青睐。目前的非制冷型长波红外探测器(例如微测辐射热计)的性能受到灵敏度降低、响应时间慢以及缺乏动态光谱可调性等因素的限制。在这里,我们利用石墨烯的可调光学和电子特性,提出了一种具有高探测率和快速响应时间的高效室温近红外探测器。与光腔耦合的图案化石墨烯上的狄拉克质子增强了固有的弱光吸收。吸收的能量在非对称载流子生成环境下通过塞贝克效应转化为光电压。此外,还通过静电门控实现了 8-12 μm 长波红外波段的动态光谱可调谐性。所提出的探测平台为新一代基于石墨烯的非致冷长波红外光探测器铺平了道路,该探测器可广泛应用于分子传感、医疗诊断、军事、安全和太空等领域。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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