Closing the nuclear fuel cycle: Strategic approaches for NuScale-like reactor

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-11-06 DOI:10.1016/j.nucengdes.2024.113672
Keferson de A. Carvalho , Graiciany Barros , Matheus H.S. Araújo , Andre A. Campagnole dos Santos , Vitor Silva , Tiago Augusto Santiago Vieira , Rebeca Cabral Gonçalves
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Abstract

The present study proposes the potential implementation of eight different closed fuel cycle strategies for a NuScale-like reactor core using its own spent fuel as a reusable source of fissile material for energy production. For that, the spent fuel composition after three burnup cycles of approximately 12 MWd/kgU of NuScale-like initial core and five years of cooling in a spent fuel pool was theoretically reprocessed by GANEX or UREX+ methods. After reprocessing, these two new fuel compositions were spiked in a mixture of thorium (Th) or depleted uranium (DpU), and afterwards inserted into specific batch positions of the core. Therefore, the proposed NuScale-like core configurations contain fuel assemblies loaded with conventional uranium-based fuel and others loaded with reprocessed fuel, resulting in the following combinations: UO2 and GANEX spiked with Th, UO2 and GANEX spiked with DpU, UO2 and UREX+ spiked with Th, UO2 and UREX+ spiked with DpU. The main idea is to comprehend the advantages of adopting the closed nuclear fuel cycle for a NuScale-like reactor by comparing the reference case and the cases containing reprocessed fuel. The results exhibited that all instances in which the core was simulated with reprocessed fuel improved the feedback coefficient, maximum excess of reactivity varying the boron concentration in the coolant, and power peak factor (PPF). Furthermore, the closed nuclear fuel strategies also demonstrated savings of about 17.50% in terms of separating work units (SWU) due to plutonium and uranium recycling, and a potential burnup extension of approximately 43%. The Serpent code version 2.1.32 developed by VTT and ENDF/B-VII.0 nuclear data library has been used to perform the simulations.
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关闭核燃料循环:类似 NuScale 反应堆的战略方法
本研究提出了对类似 NuScale 反应堆堆芯实施八种不同闭式燃料循环战略的可能性,将其自身的乏燃料作为可重复使用的裂变材料来源用于能源生产。为此,理论上采用 GANEX 或 UREX+ 方法对 NuScale 类初始堆芯经过三个燃烧周期(约 12 MWd/kgU)并在乏燃料池中冷却五年后的乏燃料成分进行后处理。后处理后,这两种新燃料成分被添加到钍(Th)或贫化铀(DpU)混合物中,然后插入堆芯的特定批次位置。因此,拟议的类似 NuScale 的堆芯配置包含装入传统铀基燃料的燃料组件和装入后处理燃料的其他组件,从而形成以下组合:二氧化铀和加有 Th 的 GANEX、加有 DpU 的二氧化铀和 GANEX、加有 Th 的二氧化铀和 UREX+、加有 DpU 的二氧化铀和 UREX+。主要想法是通过比较参考案例和含有后处理燃料的案例,了解类似 NuScale 反应堆采用封闭式核燃料循环的优势。结果表明,用后处理燃料模拟堆芯的所有情况都改善了反馈系数、冷却剂中硼浓度变化的最大反应过剩量和功率峰值因数(PPF)。此外,由于钚和铀的回收利用,封闭式核燃料策略还节省了约 17.50%的分离工作单位(SWU),并可能将燃烧时间延长约 43%。模拟使用了 VTT 开发的 Serpent 代码 2.1.32 版和 ENDF/B-VII.0 核数据图书馆。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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