Size dependent polarities in tribocharged dust aggregates.

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Soft Matter Pub Date : 2024-11-22 DOI:10.1039/d4sm01013b
Christopher Grünebeck, Florence Chioma Onyeagusi, Jens Teiser, Gerhard Wurm
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Abstract

It is long known that particles of the same material but with different sizes charge with different polarities in mutual collisions. In most cases, the smaller grains become negative. Here, we study tribocharging of (sub-)mm dust aggregates in the course of microgravity experiments by determining the charges of particles through their motion within an electric field. Similar experiments were already conducted with monolithic grains. Here, the constituent dust grains in an aggregate add complexity to the process of tribocharging in various ways. This ranges from the dust size scale, setting local surface curvatures, over shifting grains during collisions, altering the outer surfaces and potentially generating sub-surface tribocharging, to material-dependent tribocharging with a non-homogeneous dust composition. Nevertheless, in concert with the usual size dependence, the small aggregates predominantly charge negatively, the large population charges predominantly positively.

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三电荷尘埃聚集体中与尺寸相关的极性。
众所周知,相同材料但大小不同的颗粒在相互碰撞时会产生不同极性的电荷。在大多数情况下,较小的颗粒会变成负电荷。在这里,我们研究了微重力实验过程中(亚)毫米尘埃聚集体的三极电荷,通过粒子在电场中的运动来确定它们的电荷。类似的实验已经在整体颗粒上进行过。在这里,聚集体中的组成尘粒以各种方式增加了三电荷过程的复杂性。这包括尘粒的大小尺度、局部表面曲率、碰撞过程中尘粒的移动、外表面的改变和可能产生的次表面三电荷,以及非均质尘粒组成的材料三电荷。然而,与通常的尺寸依赖性一致的是,小的聚集体主要带负电荷,大的聚集体主要带正电荷。
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来源期刊
Soft Matter
Soft Matter 工程技术-材料科学:综合
CiteScore
6.00
自引率
5.90%
发文量
891
审稿时长
1.9 months
期刊介绍: Where physics meets chemistry meets biology for fundamental soft matter research.
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