Biomimetic methodology as a sustainable tool for enhanced photocatalytic reduction of CO2

IF 5.2 2区 化学 Q1 CHEMISTRY, APPLIED Catalysis Today Pub Date : 2024-11-10 DOI:10.1016/j.cattod.2024.115122
Mufeedah Muringa Kandy, Thasnim P Mohammed, Akhila George, Muniyandi Sankaralingam
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Abstract

In this current technological world, the unrestrained release of CO2 negatively impacts the atmosphere by global warming. The capture of CO2 and converting it into accessible solar fuels is a prominent scientific and technological breakthrough that tackles both the rising climate change and energy crisis issues. The dual beneficial approach focusing on solar-energy-driven reduction of CO2 to valuable energy fuels is one of the most promising sustainable strategies. In consideration of this, it has been recently observed that biomimetic strategies that incorporate intricate structural design with massive functional components offer a sustainable technological feature. Inspired by the remarkably efficient process of photosynthesis in nature, the fabrication of synthetic leaves for artificial photosynthesis emerges as an attractive avenue that addresses the dual challenges of climate change and energy scarcity with inventive and sustainable methods. This review deals with the fabrication of biomimetic materials with high surface area and efficient charge transfer mechanisms, to improve photocatalytic performance and develop sustainable solutions for CO2 capture and conversion into solar fuels. The research highlights that the current challenges hinder the advancements of the process from its nascent stage and outlines future research endeavors necessary to elevate it from a rudimentary artificial leaf concept to a commercially viable artificial tree technology with significant industrial value.
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仿生方法作为增强光催化CO2还原的可持续工具
在当今这个技术发达的世界里,二氧化碳的无限制释放会导致全球变暖,对大气产生负面影响。捕获二氧化碳并将其转化为可获取的太阳能燃料是解决日益严重的气候变化和能源危机问题的一项重大科技突破。将太阳能驱动的二氧化碳减少为有价值的能源燃料的双重有益方法是最有前途的可持续战略之一。考虑到这一点,最近观察到,将复杂的结构设计与大量功能部件相结合的仿生策略提供了一种可持续的技术特征。受自然界高效的光合作用过程的启发,人工光合作用合成叶片的制造成为解决气候变化和能源短缺双重挑战的一种有吸引力的途径,这种方法具有创造性和可持续性。本文综述了具有高表面积和高效电荷转移机制的仿生材料的制备,以提高光催化性能,并为二氧化碳捕获和转化为太阳能燃料开发可持续的解决方案。该研究强调,目前的挑战阻碍了该过程从初期阶段的进步,并概述了未来的研究努力,以将其从基本的人造叶子概念提升到具有重要工业价值的商业上可行的人造树技术。
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来源期刊
Catalysis Today
Catalysis Today 化学-工程:化工
CiteScore
11.50
自引率
3.80%
发文量
573
审稿时长
2.9 months
期刊介绍: Catalysis Today focuses on the rapid publication of original invited papers devoted to currently important topics in catalysis and related subjects. The journal only publishes special issues (Proposing a Catalysis Today Special Issue), each of which is supervised by Guest Editors who recruit individual papers and oversee the peer review process. Catalysis Today offers researchers in the field of catalysis in-depth overviews of topical issues. Both fundamental and applied aspects of catalysis are covered. Subjects such as catalysis of immobilized organometallic and biocatalytic systems are welcome. Subjects related to catalysis such as experimental techniques, adsorption, process technology, synthesis, in situ characterization, computational, theoretical modeling, imaging and others are included if there is a clear relationship to catalysis.
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