Ambipolar conduction in gated tungsten disulphide nanotube

IF 5.1 3区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Nanoscale Pub Date : 2024-12-03 DOI:10.1039/D4NR04877F
Aniello Pelella, Luca Camilli, Filippo Giubileo, Alla Zak, Maurizio Passacantando, Yao Guo, Kimberly Intonti, Arun Kumar and Antonio Di Bartolomeo
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Abstract

Devices based on transition metal dichalcogenide nanotubes hold great potential for electronic and optoelectronic applications. Herein, the electrical transport and photoresponse characteristics of a back-gate device with a channel made of a single tungsten disulfide (WS2) nanotube are investigated as functions of electric stress, ambient pressure, and illumination. As a transistor, the device exhibits p-type conduction, which can be transformed into ambipolar conduction at a high drain–source voltage. Increasing ambient pressure enhances the p-type behaviour, while exposure to light has the opposite effect, enhancing n-type conduction. The ability to operate the device as either a p-type or n-type transistor makes it promising for complementary metal–oxide–semiconductor (CMOS) circuit applications. Light enhances the conductivity, allowing for further control and enabling the device to function as a photodetector with a photoresponsivity of about 50 mA W−1 and a broadband response in the visible range. The combination of voltage, pressure and light control paves the way for using the WS2 nanotube transistor as a multifunctional device.

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门控二硫化钨纳米管的双极导电性
基于过渡金属二硫化物纳米管的器件在电子和光电子领域具有巨大的应用潜力。本文研究了由单根二硫化钨(WS2)纳米管构成的后通道器件的电输运和光响应特性作为电应力、环境压力和光照的函数。作为晶体管,该器件表现为p型导通,在高漏源极电压下可转化为双极导通。增加环境压力增强p型行为,而暴露于光有相反的效果,增强n型传导。作为p型或n型晶体管操作器件的能力使其在互补金属氧化物半导体(CMOS)电路应用中具有前景。光增强了电导率,允许进一步控制,并使该设备作为光电探测器,光响应率约为50 mA/W,在可见光范围内具有宽带响应。电压、压力和光控制的结合为WS2纳米管晶体管作为多功能器件的使用铺平了道路。
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来源期刊
Nanoscale
Nanoscale CHEMISTRY, MULTIDISCIPLINARY-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
12.10
自引率
3.00%
发文量
1628
审稿时长
1.6 months
期刊介绍: Nanoscale is a high-impact international journal, publishing high-quality research across nanoscience and nanotechnology. Nanoscale publishes a full mix of research articles on experimental and theoretical work, including reviews, communications, and full papers.Highly interdisciplinary, this journal appeals to scientists, researchers and professionals interested in nanoscience and nanotechnology, quantum materials and quantum technology, including the areas of physics, chemistry, biology, medicine, materials, energy/environment, information technology, detection science, healthcare and drug discovery, and electronics.
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