A modelling framework to analyze climate change effects on radionuclide aquifer contamination.

IF 3.5 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Journal of contaminant hydrology Pub Date : 2024-11-29 DOI:10.1016/j.jconhyd.2024.104470
Thomas Matteo Coscia, Francesco Di Maio, Enrico Zio
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Abstract

Non-stationarity of climatic variables (e.g., temperature and precipitation) due to Climate Change (CC) can affect the migration processes of radionuclides released from nuclear activities. In this paper, a framework of analysis is developed to predict the evolution in time of contaminant concentration and fluence under different Climatic Boundary Conditions (CBCs) of precipitation scenarios provided by a climate model integrated with an accurate physical coupled hydraulic-transport model. A case study is worked out with respect to the migration of a radioactive contaminant (232Th) at Kirtland Air Force Base (Albuquerque, New Mexico, USA), for which the different CBCs considered are: i) stationary and ii) non-stationary precipitation. The effects of such alternative hypotheses on the physical modelling results are analysed, using a cross-wavelet analysis. It is shown that fluence is strongly affected by precipitation extremes, more than concentration, and it is claimed that a daily scale on the information and data of CBCs is necessary to model, with sufficient accuracy, the migration process and properly assess the impact of future CC on groundwater contamination.

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分析气候变化对放射性核素含水层污染影响的模拟框架。
气候变化(CC)引起的气候变量(如温度和降水)的非平稳性可影响核活动释放的放射性核素的迁移过程。本文建立了一个分析框架,以预测不同降水情景气候边界条件(CBCs)下污染物浓度和影响的时间演变,该分析框架由气候模式与精确的物理耦合水力-输运模式相结合。在科特兰空军基地(美国新墨西哥州阿尔伯克基)对放射性污染物(232Th)的迁移进行了案例研究,其中考虑的不同CBCs是:i)固定沉淀和ii)非固定沉淀。使用交叉小波分析,分析了这些替代假设对物理模拟结果的影响。研究表明,降水极端事件对影响的影响比对浓度的影响更大,并认为有必要对CBCs的信息和数据进行日尺度的模拟,以达到足够的精度,并正确评估未来CC对地下水污染的影响。
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来源期刊
Journal of contaminant hydrology
Journal of contaminant hydrology 环境科学-地球科学综合
CiteScore
6.80
自引率
2.80%
发文量
129
审稿时长
68 days
期刊介绍: The Journal of Contaminant Hydrology is an international journal publishing scientific articles pertaining to the contamination of subsurface water resources. Emphasis is placed on investigations of the physical, chemical, and biological processes influencing the behavior and fate of organic and inorganic contaminants in the unsaturated (vadose) and saturated (groundwater) zones, as well as at groundwater-surface water interfaces. The ecological impacts of contaminants transported both from and to aquifers are of interest. Articles on contamination of surface water only, without a link to groundwater, are out of the scope. Broad latitude is allowed in identifying contaminants of interest, and include legacy and emerging pollutants, nutrients, nanoparticles, pathogenic microorganisms (e.g., bacteria, viruses, protozoa), microplastics, and various constituents associated with energy production (e.g., methane, carbon dioxide, hydrogen sulfide). The journal''s scope embraces a wide range of topics including: experimental investigations of contaminant sorption, diffusion, transformation, volatilization and transport in the surface and subsurface; characterization of soil and aquifer properties only as they influence contaminant behavior; development and testing of mathematical models of contaminant behaviour; innovative techniques for restoration of contaminated sites; development of new tools or techniques for monitoring the extent of soil and groundwater contamination; transformation of contaminants in the hyporheic zone; effects of contaminants traversing the hyporheic zone on surface water and groundwater ecosystems; subsurface carbon sequestration and/or turnover; and migration of fluids associated with energy production into groundwater.
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