Multimodality Imaging of Fluid Saturation and Chemical Transport for Two-Phase Surfactant/Polymer Floods in Porous Rocks

IF 2.7 3区 工程技术 Q3 ENGINEERING, CHEMICAL Transport in Porous Media Pub Date : 2024-12-12 DOI:10.1007/s11242-024-02146-0
Andrea Rovelli, James Brodie, Bilal Rashid, Weparn J. Tay, Ronny Pini
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Abstract

Multicomponent, two-phase flow in porous media is a problem of practical relevance that remains difficult to study experimentally. Advanced methodologies are needed that enable the monitoring of both the saturation of each fluid phase within the pore space and the concentration of the chemical species within the fluids. We present an approach based on multimodality imaging and apply it to the case study of surfactant/polymer flooding in a sandstone for enhanced oil recovery. X-ray computed tomography and positron emission tomography (PET) are applied for the asynchronous acquisition of dynamic profiles of saturations (aqueous and oleic) and of the solute concentration within the surfactant/polymer slug, respectively. This complementary dataset enables precise investigation of the evolution of both the oil bank and the induced mixing at its rear arising from the surfactant/polymer flooding process. The dilution index, intensity of segregation and the spreading length are used to quantify the degree of mixing within the surfactant/polymer slug as a function of time from the spatial structure of the solute concentration field. Relative to the single-phase flow scenario, a threefold increase in dispersivity is observed. We demonstrate that mixing is systematically overestimated if only the PET dataset is used—highlighting the importance of implementing multimodality imaging. We also show that the advection–dispersion equation model, parameterised using the dispersivity derived from the experiments, provides reasonable estimates for the rate of both mixing and spreading.

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多孔岩石中两相表面活性剂/聚合物驱流体饱和度和化学输运的多模态成像
多孔介质中的多组分两相流是一个具有实际意义的问题,但实验研究仍然很困难。需要先进的方法来监测孔隙空间内每个流体相的饱和度和流体中化学物质的浓度。我们提出了一种基于多模态成像的方法,并将其应用于砂岩表面活性剂/聚合物驱提高采收率的案例研究。x射线计算机断层扫描和正电子发射断层扫描(PET)分别用于异步获取饱和(含水和含油)和表面活性剂/聚合物段塞内溶质浓度的动态剖面。这个补充数据集可以精确地研究油库的演变以及表面活性剂/聚合物驱过程中引起的油库后部的诱导混合。从溶质浓度场的空间结构出发,利用稀释指数、偏析强度和扩散长度来量化表面活性剂/聚合物段塞内的混合程度作为时间函数。相对于单相流的情况,分散性增加了三倍。我们证明,如果只使用PET数据集,混合被系统地高估了,这突出了实现多模态成像的重要性。我们还表明,使用实验得出的色散参数化的平流-色散方程模型,对混合和扩散的速率提供了合理的估计。
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来源期刊
Transport in Porous Media
Transport in Porous Media 工程技术-工程:化工
CiteScore
5.30
自引率
7.40%
发文量
155
审稿时长
4.2 months
期刊介绍: -Publishes original research on physical, chemical, and biological aspects of transport in porous media- Papers on porous media research may originate in various areas of physics, chemistry, biology, natural or materials science, and engineering (chemical, civil, agricultural, petroleum, environmental, electrical, and mechanical engineering)- Emphasizes theory, (numerical) modelling, laboratory work, and non-routine applications- Publishes work of a fundamental nature, of interest to a wide readership, that provides novel insight into porous media processes- Expanded in 2007 from 12 to 15 issues per year. Transport in Porous Media publishes original research on physical and chemical aspects of transport phenomena in rigid and deformable porous media. These phenomena, occurring in single and multiphase flow in porous domains, can be governed by extensive quantities such as mass of a fluid phase, mass of component of a phase, momentum, or energy. Moreover, porous medium deformations can be induced by the transport phenomena, by chemical and electro-chemical activities such as swelling, or by external loading through forces and displacements. These porous media phenomena may be studied by researchers from various areas of physics, chemistry, biology, natural or materials science, and engineering (chemical, civil, agricultural, petroleum, environmental, electrical, and mechanical engineering).
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