Enhancing the NO2 detection ability of surface acoustic wave sensors with ZnO-decorated N-doped porous carbon nanosheets†

IF 5.7 2区 材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY Journal of Materials Chemistry C Pub Date : 2024-10-29 DOI:10.1039/D4TC03690E
Xue Li, Yuan Feng, Haifeng Lv, Junjie Shi, Yuanjun Guo, Sean Li and Xiaotao Zu
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Abstract

Effective detection of nitrogen dioxide (NO2) is crucial for environmental safety and human health. Gas sensors utilizing surface acoustic wave (SAW) technology hold significant promise for detecting hazardous gases, but their performance heavily depends on the intrinsic properties of the sensing layer materials. In this study, we elaborate on using ZnO nanoparticle-dispersed N-doped porous carbon nanosheets (ZnO@N-PCNs) for SAW sensors aimed at achieving rapid NO2 detection at room temperature. The resultant ZnO@N-PCNs SAW gas sensor exhibits a significant frequency shift of approximately −4.4 kHz, which is much higher than that of the pristine N-PCNs SAW sensor at a NO2 concentration of 20 ppm. It responds quickly when exposed to NO2 gas, and demonstrates specific selectivity and good reproducibility over both short and long terms. This work reveals the sensing properties of ZnO-optimized SAW sensors and provides valuable guidance for the development of high-sensitivity SAW sensors.

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有效检测二氧化氮(NO2)对环境安全和人类健康至关重要。利用表面声波(SAW)技术的气体传感器在检测有害气体方面大有可为,但其性能在很大程度上取决于传感层材料的内在特性。在本研究中,我们详细阐述了如何将 ZnO 纳米粒子分散的 N 掺杂多孔碳纳米片(ZnO@N-PCNs)用于声表面波传感器,以实现室温下的快速二氧化氮检测。在二氧化氮浓度为 20ppm 时,ZnO@N-PCNs 声表面波气体传感器的频移约为 -4.4 kHz,远高于原始 N-PCNs 声表面波传感器的频移。当暴露在二氧化氮气体中时,它能迅速做出反应,并在短期和长期内表现出特定的选择性和良好的重现性。这项研究揭示了氧化锌优化声表面波传感器的传感特性,为开发高灵敏度声表面波传感器提供了宝贵的指导。
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来源期刊
Journal of Materials Chemistry C
Journal of Materials Chemistry C MATERIALS SCIENCE, MULTIDISCIPLINARY-PHYSICS, APPLIED
CiteScore
10.80
自引率
6.20%
发文量
1468
期刊介绍: The Journal of Materials Chemistry is divided into three distinct sections, A, B, and C, each catering to specific applications of the materials under study: Journal of Materials Chemistry A focuses primarily on materials intended for applications in energy and sustainability. Journal of Materials Chemistry B specializes in materials designed for applications in biology and medicine. Journal of Materials Chemistry C is dedicated to materials suitable for applications in optical, magnetic, and electronic devices. Example topic areas within the scope of Journal of Materials Chemistry C are listed below. This list is neither exhaustive nor exclusive. Bioelectronics Conductors Detectors Dielectrics Displays Ferroelectrics Lasers LEDs Lighting Liquid crystals Memory Metamaterials Multiferroics Photonics Photovoltaics Semiconductors Sensors Single molecule conductors Spintronics Superconductors Thermoelectrics Topological insulators Transistors
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