Growth of CdZnTe crystal under high magnetic field and its photon-counting detector performance

IF 5.8 2区 材料科学 Q2 CHEMISTRY, PHYSICAL Journal of Alloys and Compounds Pub Date : 2025-01-15 DOI:10.1016/j.jallcom.2024.178390
Jiongjiong Wei , Linjun Wang , Yingdong Huang , Kun Liu , Wanping Liu , Wenxuan Yang , Xiaoyan Liang , Jijun Zhang
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Abstract

In this paper, CdZnTe (CZT) crystal was grown by the Traveling Heater Method (THM) under 5 T axial static magnetic field, which improved the quality of CZT crystal and the performance of photon-counting detector. The effect of high magnetic field on the quality of CZT crystal and the mechanism of internal defects were experimentally studied. The concentration of Te inclusions in CZT crystals grown by THM under high magnetic field was about 5 × 103 /cm3 with the size less than 5μm observed by infrared microscope, which were one order of magnitude lower than those grown without magnetic field. Then the planar CZT detector was fabricated to study the photoelectric properties of CZT crystals grown by THM. The resistivity of CZT under high magnetic field was 2.83 × 1010Ω·cm, and its energy resolution to 241Am (59.5 keV) was 5.9 %. The photocurrent maintained a good linearity under the tube current of 0.1mA-0.6 mA during the photocurrent response test. The results indicate that the detector prepared by CZT crystal grown under high magnetic field is better than that grown without magnetic field. Finally, the CZT wafers were made into 1 × 16 linear-array pixel detectors with a pixel size of 0.9 × 1.8 mm2. The photon-counting rate and imaging quality of the CZT linear array detector under X-ray irradiation were studied. The average saturated photon-counting rate reached 2.0 × 106 CPS/Channel (Counts Per Second/Channel).

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高磁场下CdZnTe晶体的生长及其光子计数探测器性能
本文在5t轴向静态磁场下,采用行热法生长CdZnTe (CZT)晶体,提高了CZT晶体的质量和光子计数探测器的性能。实验研究了强磁场对CZT晶体质量的影响及内部缺陷的形成机理。高磁场下THM生长的CZT晶体中Te夹杂物的浓度约为5×103 /cm3,尺寸小于5μm的CZT晶体中Te夹杂物的浓度比无磁场生长的CZT晶体低一个数量级。然后制作平面型CZT探测器,研究THM生长的CZT晶体的光电特性。高磁场下CZT的电阻率为2.83×1010Ω·cm, 241Am (59.5 keV)的能量分辨率为5.9%。在光电流响应测试中,在0.1mA-0.6 mA的管电流下,光电流保持良好的线性。结果表明,在强磁场下生长的CZT晶体制备的探测器比在无磁场下生长的要好。最后,将CZT晶圆制成像素尺寸为0.9×1.8 mm2的1×16线性阵列像素探测器。研究了x射线辐照下CZT线阵探测器的光子计数率和成像质量。平均饱和光子计数率达到2.0×106 CPS/Channel (Counts Per Second/Channel)。
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来源期刊
Journal of Alloys and Compounds
Journal of Alloys and Compounds 工程技术-材料科学:综合
CiteScore
11.10
自引率
14.50%
发文量
5146
审稿时长
67 days
期刊介绍: The Journal of Alloys and Compounds is intended to serve as an international medium for the publication of work on solid materials comprising compounds as well as alloys. Its great strength lies in the diversity of discipline which it encompasses, drawing together results from materials science, solid-state chemistry and physics.
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