A general strategy to achieve see-through devices through the micro-structuring of colored functional materials.

IF 15.7 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES Nature Communications Pub Date : 2024-12-30 DOI:10.1038/s41467-024-55133-w
Zishou Hu, Xueqing Tang, Yuan-Qiu-Qiang Yi, Shuhong Nie, Xiaolian Chen, Wenya Xu, Chenchao Huang, Xinju Mu, Zhongsheng Ma, Pengyu Tang, Xinzhou Wu, Wenming Su, Christine K Luscombe
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Abstract

Irrespective of the specific see-through device, obtaining optimal transparency remains the primary goal. In this work, we introduce a general strategy to enhance the transparency of various see-through devices. We achieve this by structuring the colored functional materials into imperceptible three-dimensional mesh lines, addressing a common challenge in multi-layer structures where each layer causes a reduction in transparency due to their color or opacity. To overcome this limitation, we selectively integrate functional materials into micron-wide groove structures transforming functional layers to functional meshes. Regardless of the initial color of the functional material, the resulting functional mesh can exhibit a high transmittance of 88% (vs. air) under any operating state while maintaining its intended function within the device. We apply this strategy to fabricate proof-of-concept of devices such as electrochromic devices, supercapacitors, and zinc batteries, all of which exhibit remarkable overall transparency when compared to the multi-layer device.

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通过有色功能材料的微结构实现透明器件的一般策略。
不考虑具体的透明装置,获得最佳的透明度仍然是首要目标。在这项工作中,我们介绍了提高各种透明器件透明度的一般策略。我们通过将有色功能材料结构成难以察觉的三维网格线来实现这一目标,解决了多层结构中的常见挑战,其中每层由于其颜色或不透明度而导致透明度降低。为了克服这一限制,我们选择性地将功能材料集成到微米宽的凹槽结构中,将功能层转化为功能网格。无论功能材料的初始颜色如何,所得到的功能网格在任何工作状态下都可以表现出88%(相对于空气)的高透光率,同时在设备内保持其预期功能。我们将此策略应用于制造概念验证器件,如电致变色器件,超级电容器和锌电池,与多层器件相比,所有这些器件都具有显着的整体透明度。
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阿拉丁
2,2-dimethoxy-2-phenylacetophenone (DMPAP)
阿拉丁
Poly(ethylene glycol) diacrylate (PEGDA)
阿拉丁
Polyethylenimine (PEI)
阿拉丁
Boric acid (H3BO3)
阿拉丁
Sodium sulfate (Na2SO4)
阿拉丁
Zinc acetate (ZnAc2)
阿拉丁
Zinc chloride (ZnCl2)
阿拉丁
Zinc sulfate (ZnSO4)
阿拉丁
Lithium bromide (LiBr)
阿拉丁
Lithium perchlorate (LiClO4)
阿拉丁
Hydrogen peroxide
阿拉丁
Tungsten powder
阿拉丁
2,2-dimethoxy-2-phenylacetophenone (DMPAP)
阿拉丁
Poly(ethylene glycol) diacrylate (PEGDA)
阿拉丁
Polyethylenimine (PEI)
阿拉丁
Boric acid (H3BO3)
阿拉丁
Sodium sulfate (Na2SO4)
阿拉丁
Zinc acetate (ZnAc2)
阿拉丁
Zinc chloride (ZnCl2)
阿拉丁
Zinc sulfate (ZnSO4)
阿拉丁
Lithium bromide (LiBr)
阿拉丁
Lithium perchlorate (LiClO4)
阿拉丁
Hydrogen peroxide
阿拉丁
Tungsten powder
来源期刊
Nature Communications
Nature Communications Biological Science Disciplines-
CiteScore
24.90
自引率
2.40%
发文量
6928
审稿时长
3.7 months
期刊介绍: Nature Communications, an open-access journal, publishes high-quality research spanning all areas of the natural sciences. Papers featured in the journal showcase significant advances relevant to specialists in each respective field. With a 2-year impact factor of 16.6 (2022) and a median time of 8 days from submission to the first editorial decision, Nature Communications is committed to rapid dissemination of research findings. As a multidisciplinary journal, it welcomes contributions from biological, health, physical, chemical, Earth, social, mathematical, applied, and engineering sciences, aiming to highlight important breakthroughs within each domain.
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