Design of a graphene-based chiral trifunctional tunable terahertz metasurface

IF 2.9 3区 化学 Q3 CHEMISTRY, PHYSICAL Physical Chemistry Chemical Physics Pub Date : 2025-01-09 DOI:10.1039/D4CP04423A
Kun Hu, Yunpeng Yao, Lipengan Ye, Zongli Hu, Bin Tang and Wei Su
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Abstract

Driven by the pressing demand for integration and miniaturization within the terahertz (THz) spectrum, this research introduces an innovative approach to construct chiral structures using dichroism as the target function. This initiative aims to tackle the prevalent issues of single-functionality, narrow application scope, and intricate design in conventional metasurfaces. The proposed multifunctional tunable metasurface employs a graphene-metal hybrid structure to address the critical constraints found in existing designs. When circularly polarized light is incident, the metasurface exhibits broadband circular dichroism (CD) function, generating CD intensities greater than 0.5 at 3.44–6.0 THz, and polarization switching function at 3.43–6.17 THz. When linearly polarized light is incident, the proposed design exhibits a broadband linear dichroism (LD) function, producing LD intensities greater than 0.5 at 2.25–5.65 THz and a polarization conversion function at 3.32–6.05 THz. Its broad bandwidth ensures that each function is competitive and effective. A noteworthy feature is the capability to adjust the graphene's chemical potential and the state of the incident light to finely calibrate the intensity of each functional aspect. This innovation makes the proposed multifunctional metasurface a significant reference for the development of chiral photodetectors, CD supermirrors, smart switches, and polarization digital imaging systems within the THz range.

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基于石墨烯的手性三功能可调谐太赫兹超表面的设计
在太赫兹(THz)频谱内集成化和小型化的迫切需求驱动下,本研究提出了一种以二向性为目标函数构建手性结构的创新方法。该计划旨在解决传统元表面中普遍存在的单一功能、狭窄的应用范围和复杂的设计问题。所提出的多功能可调谐超表面采用石墨烯-金属混合结构来解决现有设计中的关键限制。当圆偏振光入射时,超表面表现出宽带圆二色性(CD)功能,在3.44 ~ 6.0 THz处产生CD强度大于0.5,在3.43 ~ 6.17 THz处产生偏振开关功能。当线偏振光入射时,所提出的设计显示出宽带线性二色性(LD)函数,在2.25-5.65太赫兹处产生大于0.5的LD强度,在3.32-6.05太赫兹处产生偏振转换函数。它的宽频带确保了每个功能都具有竞争性和有效性。一个值得注意的特点是能够调整石墨烯的化学势和入射光的状态,以精细地校准每个功能方面的强度。这一创新使得所提出的多功能超表面为开发手性光电探测器、CD超镜、智能开关和太赫兹范围内的偏振数字成像系统提供了重要的参考。
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来源期刊
Physical Chemistry Chemical Physics
Physical Chemistry Chemical Physics 化学-物理:原子、分子和化学物理
CiteScore
5.50
自引率
9.10%
发文量
2675
审稿时长
2.0 months
期刊介绍: Physical Chemistry Chemical Physics (PCCP) is an international journal co-owned by 19 physical chemistry and physics societies from around the world. This journal publishes original, cutting-edge research in physical chemistry, chemical physics and biophysical chemistry. To be suitable for publication in PCCP, articles must include significant innovation and/or insight into physical chemistry; this is the most important criterion that reviewers and Editors will judge against when evaluating submissions. The journal has a broad scope and welcomes contributions spanning experiment, theory, computation and data science. Topical coverage includes spectroscopy, dynamics, kinetics, statistical mechanics, thermodynamics, electrochemistry, catalysis, surface science, quantum mechanics, quantum computing and machine learning. Interdisciplinary research areas such as polymers and soft matter, materials, nanoscience, energy, surfaces/interfaces, and biophysical chemistry are welcomed if they demonstrate significant innovation and/or insight into physical chemistry. Joined experimental/theoretical studies are particularly appreciated when complementary and based on up-to-date approaches.
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